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Rapid multiple-quantum three-dimensional fluorescence spectroscopy disentangles quantum pathways

Authors :
Stefan Mueller
Julian Lüttig
Pavel Malý
Lei Ji
Jie Han
Michael Moos
Todd B. Marder
Uwe H. F. Bunz
Andreas Dreuw
Christoph Lambert
Tobias Brixner
Source :
Nature Communications, Vol 10, Iss 1, Pp 1-11 (2019)
Publication Year :
2019
Publisher :
Nature Portfolio, 2019.

Abstract

Multidimensional spectroscopic tools are important to explore the details of molecular dynamics. Here the authors use shaped pulses to demonstrate a 3D fluorescence spectroscopy method to extract the fourth and higher-order nonlinear responses in light-molecule interaction.

Subjects

Subjects :
Science

Details

Language :
English
ISSN :
20411723
Volume :
10
Issue :
1
Database :
Directory of Open Access Journals
Journal :
Nature Communications
Publication Type :
Academic Journal
Accession number :
edsdoj.98583cda3e24488fbcad4794ccc11ec2
Document Type :
article
Full Text :
https://doi.org/10.1038/s41467-019-12602-x