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Coherent structural trapping through wave packet dispersion during photoinduced spin state switching

Authors :
Henrik T. Lemke
Kasper S. Kjær
Robert Hartsock
Tim B. van Driel
Matthieu Chollet
James M. Glownia
Sanghoon Song
Diling Zhu
Elisabetta Pace
Samir F. Matar
Martin M. Nielsen
Maurizio Benfatto
Kelly J. Gaffney
Eric Collet
Marco Cammarata
Source :
Nature Communications, Vol 8, Iss 1, Pp 1-8 (2017)
Publication Year :
2017
Publisher :
Nature Portfolio, 2017.

Abstract

Ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remain challenging to describe since electronic/nuclear configurations are coupled. Here the authors use time-resolved X-ray absorption spectroscopy to probe the light-induced spin-state trapping dynamics of [Fe(bpy)3]2+beyond the Born-Oppenheimer approximation.

Subjects

Subjects :
Science

Details

Language :
English
ISSN :
20411723
Volume :
8
Issue :
1
Database :
Directory of Open Access Journals
Journal :
Nature Communications
Publication Type :
Academic Journal
Accession number :
edsdoj.f550e3664db64b8489fa20caa1ce88e4
Document Type :
article
Full Text :
https://doi.org/10.1038/ncomms15342