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Dual-stimuli responsive photonic barcodes based on perovskite quantum dots encapsulated in whispering-gallery-mode microspheres
- Source :
- Journal of Materiomics, Vol 9, Iss 3, Pp 423-430 (2023)
- Publication Year :
- 2023
- Publisher :
- Elsevier, 2023.
-
Abstract
- Micro/nanoscale photonic barcodes hold great potential for broad applications in items tracking, multiplexed bioassays and anti-counterfeiting. The ever-increasing demand in advanced anti-counterfeiting applications calls for micro/nanoscale barcodes with accurate recognition, large encoding capacity and high security level. Here, we proposed a strategy to construct the dual-stimuli responsive photonic barcodes based on the perovskite quantum dots (PQDs) doped polymer whispering-gallery-mode (WGM) microcavities via swelling-deswelling method. Benefiting from the well-defined spherical microcavities, the photoluminescence (PL) spectra of as-prepared composites exhibit a series of sharp peaks characteristics resulting from the effective WGM modulation, which constitutes the fingerprint of a specific resonator and thus allows a definition of photonic barcodes. On this basis, we achieved responsive photonic barcodes based on the volatile polar-solvent-controlled luminescence in the microspheres benefitting from the space-confined microcavities and the ionic feature of the PQDs. Moreover, the light-controlled photonic barcodes have further been acquired through reversibly regulating the inactivation and activation of the energy transfer (ET) process between the PQDs and photochromic dyes. The well-established protocols of PQDs@WGM enable the development of distinct responsive barcodes with multi-responsive features, which will pave an avenue to new types of flexible WGM-based components for optical data recording and security labels.
Details
- Language :
- English
- ISSN :
- 23528478
- Volume :
- 9
- Issue :
- 3
- Database :
- Directory of Open Access Journals
- Journal :
- Journal of Materiomics
- Publication Type :
- Academic Journal
- Accession number :
- edsdoj.f715f8c991d0487981eda035022b04d0
- Document Type :
- article
- Full Text :
- https://doi.org/10.1016/j.jmat.2022.12.009