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Zirconoarylation of alkynes through p-chloranil-promoted reductive elimination of arylzirconates

Authors :
Xiaoyu Yan
Chao Chen
Chanjuan Xi
Source :
Beilstein Journal of Organic Chemistry, Vol 10, Iss 1, Pp 528-534 (2014)
Publication Year :
2014
Publisher :
Beilstein-Institut, 2014.

Abstract

A novel method for the zirconoarylation of alkynes was developed. TCQ-promoted reductive elimination of arylzirconate [LiCp2ZrAr(RC≡CR)], which was prepared by the reaction of zirconocene–alkyne complexes with aryllithium compounds, afforded trisubstituted alkenylzirconocenes. This reaction can afford multi-substituted olefins with high stereoselectivity.

Details

Language :
English
ISSN :
18605397
Volume :
10
Issue :
1
Database :
Directory of Open Access Journals
Journal :
Beilstein Journal of Organic Chemistry
Publication Type :
Academic Journal
Accession number :
edsdoj.f72b5d74c249ca8d9945dde52f4229
Document Type :
article
Full Text :
https://doi.org/10.3762/bjoc.10.48