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Ultrafast dynamics of the SO2(H2O)(sub n) cluster system

Authors :
Dermota, T.E.
Hydutsky, D.P.
Bainco, N.J.
Castleman, A.W., Jr.
Source :
Journal of Physical Chemistry A. Sept 22, 2005, Vol. 109 Issue 37, p8254, 5 p.
Publication Year :
2005

Abstract

An investigation of the excited-state dynamics of SO2(H2O)(sub n) clusters following excitation by ultrafast laser pulses to 4.7 eV and 9.3 eV is presented. A lack of cluster size dependence in the measured time constants indicates surface solvation of SO2 rather than a cluster structure with the SO2 molecule fully encompassed by water molecules.

Subjects

Subjects :
Sulfur dioxide -- Chemical properties
Sulfur dioxide -- Optical properties
Excited state chemistry -- Research
Laser pulses, Ultrashort -- Usage
Chemicals, plastics and rubber industries

Details

Language :
English
ISSN :
10895639
Volume :
109
Issue :
37
Database :
Gale General OneFile
Journal :
Journal of Physical Chemistry A
Publication Type :
Academic Journal
Accession number :
edsgcl.141017866

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