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Magnetic properties of high-nuclearity spin clusters. Fourteen- and fifteen-oxovanadium (IV) clusters

Authors :
Barra, Anne-Laure
Gatteschi, Dante
Pardi, Luca
Muller, Achim
Doring, Joachim
Source :
Journal of the American Chemical Society. Oct 21, 1992, Vol. 114 Issue 22, p8509, 6 p.
Publication Year :
1992

Abstract

A study was done on the magnetic properties of K6(V15As6O42(H2O)). 8H2O(V15) and (NH4)6(V14As8O42(SO3))(V14) using variable-temperature magnetic susceptibility, EPR spectra and Huckel calculations. It was shown that the compound containing 15 vanadium ions has a unique multilayer structure whose magnetic properties were identified together with that of the coumpound having 14 vanadium ions. The magnetic properties of the high-nuclearity spin clusters can be elucidated using a perturbation and full matrix approach with spin hamiltonian formalism.

Details

ISSN :
00027863
Volume :
114
Issue :
22
Database :
Gale General OneFile
Journal :
Journal of the American Chemical Society
Publication Type :
Academic Journal
Accession number :
edsgcl.14242566