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Static and dynamic magnetoelastic properties of spin ice

Authors :
Wosnitza, Joachim
Geck, Jochen
Technische Universität Dresden
Stöter, Thomas
Wosnitza, Joachim
Geck, Jochen
Technische Universität Dresden
Stöter, Thomas
Publication Year :
2019

Abstract

The concept of magnetic frustration is a fundamental topic in modern solid-state physics having direct consequences in systems with rich magnetic phases hosting emergent excitations, such as the magnetic monopoles in the spin-ice compounds. One important ingredient of frustration is the lattice that constrains the magnetic spins on it to a site anisotropy and inter-site coupling. Therefore, strong magnetoelastic interactions between the magnetic system and the lattice are expected and investigated in this thesis in detail. At first, I investigate the dependence of the relative length change of single crystals of the classical spin ices \dto{} and \hto{} on the magnetic field and temperature by capacitive dilatometry. In terms of the magnetostriction and thermal expansion \dto{} and \hto{} show qualitatively similar behavior, that seems to be independent of the Kramer or non-Kramers character of the rare-earth ion. The magnitude of the magnetostrictive effect deep in the spin-ice phase at \SI{0.3}{\kelvin} is $\deltaL{} = \SI{2e-5}{}$ and $\SI{2e-4}{}$ for \dto{} and \hto{}, respectively. In numerical simulations using a manifold model, the experimental results could be qualitatively reproduced by a combination of exchange and crystal-field striction. A second highlight of the dilatometric measurements of the spin-ice compounds is the observation of the lattice dynamics. The relaxation processes are rather slow, the longest relaxation times were observed at lowest temperatures and in the field range with magnetostrictive hysteresis, \ie{}, below \SI{0.9}{\tesla} for \dto{} and below \SI{1.5}{\tesla} for \hto{}. I find that the region of longest relaxation coincides well with the kagome-ice phase of the magnetic phase diagrams; the laxation time is of the order of \SI{5000}{\second} ($> \SI{80}{\minute}$). With increasing temperatures the time scale of the relaxation reduces to minutes at around \SI{0.7}{\kelvin} corresponding to the spin-freezing temperature obtained

Details

Database :
OAIster
Notes :
English
Publication Type :
Electronic Resource
Accession number :
edsoai.on1135785974
Document Type :
Electronic Resource