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The dynamics of the neutral atoms in Hall thrusters affects several plasma processes, from ionization to electrons' mobility. In the context of Hall thruster's particle-in-cell (PIC) modeling, the neutrals are often treated kinetically, similar to the plasma species, and their interactions with themselves and the ions are resolved using the direct-simulation Monte–Carlo (DSMC) algorithm. However, the DSMC approach is computationally resource demanding. Therefore, modeling the neutrals as a 1D fluid has been also pursued in simulations that do not involve the radial coordinate and, hence, do not resolve the neutrals' radial expansion. In this article, we present an extensive study on the sensitivity of the PIC simulations of Hall thruster discharge to the model used for the neutral dynamics. We carried out 1D axial PIC simulations with various fluid and kinetic models of the neutrals as well as self-consistent quasi-2D axial-azimuthal simulations with different neutrals' fluid descriptions. Our results show that the predictions of the simulations in either 1D or 2D configurations are highly sensitive to the neutrals' model, and that different treatments of the neutrals change the spatiotemporal evolution of the discharge. Moreover, we observed that considering the ion-neutral collisions causes a significant variation in the neutral temperature, thus requiring that the neutrals' energy equation to be included as well in their fluid system of equations. Finally, the self-consistent axial-azimuthal simulations highlighted that a neutrals' model based on the continuity conservation equation only is not an appropriate choice and leads to physically unexpected high-frequency global discharge oscillations. [ABSTRACT FROM AUTHOR]

This report describes an investigation by experimentation to elucidate atmospheric discharge plasma induced using a 50 kW millimeter-wave beam at 94 GHz. Millimeter-wave discharge plasma is useful for an ultraviolet light source, radioactive material detection, chemical decomposition, and beamed energy propulsion (BEP). The gyrotron used in this study is the "UT-94" with a frequency of 94 GHz and an output power of 100 kW, which was developed at the University of Tokyo specifically for BEP research. The 94 GHz frequency is promising for atmospheric energy beaming because of its low atmospheric attenuation, small beam divergence, and existing utilization track records in the atmosphere. This study experimentally investigated the relationship between the incident beam power density and propagation velocity of an ionization-wave front, which is particularly critical to thrust performance. In addition, the plasma structures were also clarified at 94 GHz and compared with other microwave and millimeter-wave frequencies, such as 28 GHz and those higher than 100 GHz. As a result, finer microscopic structure in the H–k plane was observed than those reported in earlier studies. Furthermore, we found a clear relation between structures and propagation velocities in terms of the electric field concentration of the incoming electromagnetic-waves. [ABSTRACT FROM AUTHOR]

In recent years, interest in striation phenomena in radio frequency (rf) discharges has risen due to the availability of new experimental data and the implementation of new computational models. Depending on the conditions, different mechanisms of discharge striations are realized. These are the ionization instability, the instability due to the electron attachment to electronegative gases, or the instability due to thermoelectric transport. Although the first two mechanisms were modeled quite extensively in recent years, the understanding of the influence of the Dufour effect originating from plasma density gradients on the stability of radio frequency discharges in long tubes remains poor. In this paper, the influence of this mechanism on the longitudinal striations of radio frequency discharge is presented using a one-dimensional model of argon discharge driven with rf excitation under intermediate pressure conditions of 0.5 Torr. It is found that striation formation is sensitive to the value of the thermoelectric heat transport coefficient in the low electron temperature range. The critical value of this coefficient necessary for the instability onset is derived using the linear stability analysis. [ABSTRACT FROM AUTHOR]

We demonstrate similarity-based scaling networks for capacitive radio frequency (RF) plasmas, which extensively correlate discharge characteristics under varied conditions, incorporating the transition from original to similarity states. Based on fully kinetic particle-in-cell simulations, similar RF discharges in argon are demonstrated with three external control parameters (gas pressure, gap distance, and driving frequency) simultaneously tuned. A complete set of scaling pathways regarding fundamental discharge parameters is obtained, from which each plasma state finds its neighboring node with only one control parameter tuned. The results from this study provide a promising strategy for plasma multi-parameter mapping, enabling effective cross-comparisons, prediction, and manipulation of RF discharge plasmas. [ABSTRACT FROM AUTHOR]

The effect of driving frequency in the range of 13.56–73 MHz on electron energy distribution and electron heating modes in a 50 mTorr capacitively coupled argon plasma discharge is studied using 1D-3V particle-in-cell simulations. Calculated electron energy probability functions exhibit three distinct "temperatures" for low-, mid-, and high-energy electrons at all the studied driving frequencies. When compared to published experimental data, the calculated probability functions show a reasonable agreement for the energy range resolved in the measurements (about 2–10 eV). Discrepancies due to limitations in experimental energy resolution outside this range lead to differences between computational and experimental values of the electron number density determined from the distribution functions, and the predicted effective electron temperature is within 25% of experimental values. The impedance of the discharge is interpreted in terms of a homogeneous equivalent circuit model, and the driving frequency dependence of the inferred combined sheath thickness is found to obey a known, theoretically derived, power law. The average power transferred from the field to the electrons (electron heating) is computed, and a region of negative heating near the sheath edge, particularly at higher driving frequencies, is identified. Analysis of the electron momentum equation shows that electron inertia, which on temporal averaging would be zero in a linear regime, is responsible for negative values of power deposition near the sheath edge at high driving frequencies due to the highly nonlinear behavior of the discharge. [ABSTRACT FROM AUTHOR]

Plasma asymmetry generation in capacitively coupled plasma (CCP) discharges provides control over vital parameters that are useful in many plasma processing applications. In this article, using the particle-in-cell simulation technique, we investigated the spatial plasma asymmetry creation by a temporally asymmetric (sawtooth) waveform by varying its number of harmonics (N). The simulation results predict a non-linear increase in the plasma density and ion flux with an increase in N, i.e., it first decreases, reaching to a minimum value for a critical value of N and then increases almost linearly with a further rise in N. The ionization asymmetry increases with N, and higher harmonics on the instantaneous sheath position are observed for higher values of N. These higher harmonics generate multiple ionization beams that are generated near the expanding sheath edge and are responsible for an enhanced plasma density. The ion energy distribution function (IEDF) depicts a bi-modal shape for different values of N. DC self-bias is observed on the powered electrode, its magnitude with respect to the plasma potential decreases with increasing N, and therefore, the corresponding ion energy on the powered electrode decreases. The results conclude that by changing N of a sawtooth waveform in a collisionless CCP system, the ion flux asymmetry is not altered, whereas sheath symmetry could be significantly affected causing a systematic variation in the ion energy asymmetry. Due to an increase in the higher harmonic contents in the sawtooth waveform, a transition from broad bi-modal to narrow-shaped IEDFs is found. [ABSTRACT FROM AUTHOR]

In this paper, we discuss a number of problems found in the literature related to experimental measurements of rf discharge electrical and plasma parameters with different electromagnetic probes. Incorrect evaluations of discharge power and the inaccurate measurement of basic plasma parameters with electrical (Langmuir), magnetic (B-dot), and microwave probes are among the troubling issues found in many recent publications on rf plasma. The purpose of this review is to show the origination of errors and ways to their mitigation based on the three-decade development of contemporary rf discharge diagnostics. [ABSTRACT FROM AUTHOR]

This study analyzes the dependence of electron extraction efficiency, which is defined as the ratio of the extracted electron current to the generated electron current, on the orifice shapes and magnetic fields of a miniature microwave discharge xenon neutralizer via three-dimensional particle-in-cell simulations with Monte Carlo collisions (PIC–MCCs). The PIC–MCC simulation results show that the orifice shapes do not significantly affect the discharge characteristics or the electron extraction efficiency. However, the efficiency achieves a 1.5-times higher value in a new magnetic field configuration, referred to as MF-2, where the magnetic field lines pass through nearly the entire area of the orifices. This improvement is attributed to the reduction in the electron backflow and the electron loss toward both the downstream inside surface and the outside wall of the discharge chamber. In addition, there are relatively small plasma fluctuations in the discharge chamber for MF-2 due to its low Bohm diffusion coefficient, where no rotating spokes, which are often seen in other E × B devices, are observed. As a result, the electron loss toward the downstream surface inside the discharge chamber is reduced, and this decrease in the electron loss also contributes to the increase in the extraction efficiency. [ABSTRACT FROM AUTHOR]

This article reports experimental observation of rotating plasma discharges in a coaxial structure at a frequency of 2.45 GHz and under atmospheric pressure. In contrast to other cases, the discharge in our case spins without external static magnetic field or moving electrodes. Its formation and impact factors are experimentally explored. Results show that the rotating discharge, especially the peculiarities of its rotation velocity, is attributed to the combined action of gas flow and electromagnetic field intensity between the conductors. Raising the electromagnetic field intensity or reducing the gas flow rate in appropriate ranges can result in a notable increase of the rotation speed. Experiments also demonstrate that the rotation properties are independent of the coaxial dimensions. This article is supposed to provide a new thinking and guidelines for inducing rotating discharge in a coaxial structure without electrodes moving or external magnetic field. [ABSTRACT FROM AUTHOR]

A microwave plasma generator (MPG) of a sub-millimeter scale might be suitable for biomedical applications. However, there are still many unknowns regarding the MPG discharge behavior at this scale and specific conditions. A two-dimensional MPG model at the millimeter scale and its simulation and relative calculation in the COMSOL Multiphysics software are presented. A MPG filled with argon and helium is simulated, respectively. The frequency of a microwave source of about 5 GHz is considered. The number density and temperature of electrons as well as chemical composition are obtained at different power and pressure conditions. The electron density peaks slightly downstream of the crossing point, and the electron density is slightly asymmetrically in the y-plane due to the fact that the electromagnetic waves are absorbed asymmetrically. The electron temperature is relatively low everywhere, in part, due to the high operating pressure. The electron temperature peaks directly underneath the wave guide where the wave is absorbed. The electron density increases with the increase in the internal pressure and the input power of the MPG, the electron temperature decreases with the increase in the internal pressure of the MPG, but the electron temperature cannot be affected by the input power change of MPG. The amount of excited Ar+ and Ars (metastable atom) increases with the increase in the input power and pressure of MPG, but the amount of excited Ar almost remained unchanged. In addition, the amount of excited He almost remained unchanged, while the amount of excited He+, Hes (metastable atom), and He2+ increased with the increase in the input power and pressure of MPG. The simulation results of this model are thus informative for understanding the physical characteristics of millimeter-sized MPG, and it will provide a solid basis for the future development of such hardware in small plasma capsules for cancer therapy. [ABSTRACT FROM AUTHOR]

Biogas production is an important component of an environmentally benign renewable energy strategy. However, the cost-effectiveness of biogas production from biomass is limited by the presence of polymeric structures, which are recalcitrant to digestion by bacteria. Therefore, pretreatments must often be applied prior to anaerobic fermentation to increase yields of biogas. Many physico-chemical pretreatments have a high energy demand and are generally costly. An alternative could be the ignition of a plasma directly in the biomass substrate. The reactive species that are generated by plasma–liquid interactions, such as hydroxyl radicals and hydrogen peroxides, could contribute significantly to the disintegration of cell walls and the breakage of poorly digestible polymers. With respect to economic, processing, and other potential benefits, a microwave instigated and sustained plasma was investigated. A microwave circuit transmitted 2-kW pulses into a recirculated sodium carboxymethyl cellulose solution, which mimicked the rheological properties of biomass. Each microwave pulse had a duration of 12.5 ms and caused the ignition of a discharge after a vapor bubble had formed. Microwaves were absorbed in the process with an efficiency of ∼97%. Slow-motion imaging showed the development of the discharge. The plasma discharges provoked a decrease in the viscosity, probably caused by the shortening of polymer chains of the cellulose derivative. The decrease in viscosity by itself could reduce processing costs and promotes bacterial activity in actual biomass. The results demonstrate the potential of microwave in-liquid plasma discharges for the pretreatment of biomass. [ABSTRACT FROM AUTHOR]

A high efficiency of power coupling from the incident microwave to the discharge is a general demand for large-scale and high-power applications of microwave plasma torches. This paper aims to experimentally explore the possibility of improving the power coupling efficiency by choosing a proper glass tube in a microwave plasma torch with a metallic enclosure, rather than using additional tuning measures such as a movable short-circuited ending plunger or a three-stub tuner. The power coupling efficiencies for the glass tubes with different wall thicknesses were experimentally measured under different incident microwave powers and different pressures. The results showed that the power coupling efficiency was improved with the increase in the glass tube wall thickness in a wide range of operating conditions for the microwave plasma torch with specific dimensions. An efficiency higher than 85% can be achieved once the wall thickness of the glass tube is in a particular range. This indicates that external tuning measures can be reduced for the microwave plasma torch with a proper glass tube, which helps to save the cost of tuning devices and enhance the flexibility in different working environments. [ABSTRACT FROM AUTHOR]

During the initial phase of microwave (MW) power launch inside a MW discharge ion source (MDIS), plasma and the total electric field (MW and ambipolar) are evolved with time together in the volume. In the presence of a plasma gradient, an ambipolar electric field is generated which interacts with the MW electric field forming a resultant total electric field which continuously varies during this evolution period. The spatio-temporal evolution pattern inside the MDIS volume is reported here, highlighting the role of the total electric field in power coupling processes. The Finite Element Method (FEM) is used to calculate the evolutions of the electric field and power coupling processes. Unlike a Particle-in-cell/Monte Carlo collision or a hybrid fluid, here, the FEM model uses time dependent Poisson solver through the drift-diffusion approach. It is observed that the main power coupling mechanism is the electron cyclotron resonance (ECR) method; however with the evolution of plasma, the mode shifts from ECR to off-ECR type heating with time. Off-ECR heating in the form of the upper-hybrid resonance method and the electrostatic ion acoustic wave heating method are two important heating mechanisms during the over-dense plasma condition, when the plasma density is above the critical density for a launched MW frequency, 2.45 GHz. In addition, the shifting of heating mechanisms from ECR to off-ECR methods is discussed based on the 3D maps of spatio-temporal evolution of plasma density and hot electron temperature. Furthermore, simulated temporal hot electron temperature and plasma density values are validated with the experiment under a similar configuration and an operating environment. [ABSTRACT FROM AUTHOR]

Several experiments have shown that the insertion of insulator materials within the plasma chamber may lead to a general improvement of microwave discharge ion source performances. In particular, the insertion of alumina into the chamber walls and borum nitride into extraction and injection flanges permits to increase the extracted current and the proton fraction and leads to a general decrease in the beam ripple. These beneficial effects have been usually explained by considering the secondary electron emission of insulators hit by plasma electrons. This paper tries to illustrate that these effects can be explained by taking into account the modification of the diffusion regime induced by the insulator materials. This approach will be used to comment on the results obtained with the versatile ion source by changing the wall conditions. [ABSTRACT FROM AUTHOR]

The problem of generating a stationary electric field in a magnetized radio-frequency discharge (rf) plasma is studied experimentally. Helmholtz coils produce magnetic field in a cylindrical vacuum chamber with diameter of 85.6 cm and length of 220 cm. RF discharge is generated at a frequency of ~5 MHz. The rf power absorbed by plasma lies in the range 0.5-1.5 kW. Electrodes defining a negative potential are placed at the ends of the chamber. Two pairs of circular flat electrodes with diameter of 5.5 and 45 cm are investigated. The working gas is argon. Radial profiles of electron density and temperature are obtained. Radial profile of the plasma potential is investigated, as well as the dependence of plasma potential on the voltage applied to the end-electrodes. [ABSTRACT FROM AUTHOR]

The reactive nitrogen-carbon plasma generated by electron cyclotron resonance (ECR) microwave discharge of N2 gas and pulsed laser ablation of a graphite target was characterized spectroscopically by time-integrated and time-resolved optical emission spectroscopy with space resolution for a study of gas-phase reactions and molecular radical formation in the plasma. The plasma exhibits very high reactivity compared with the plasma generated solely by ECR discharge or by pulsed laser ablation and contains highly excited species originally present in the ambient gaseous environment and directly ablated from the target as well as formed as the products of gas-phase reactions occurring in the plasma. The space distribution and the time evolution of the plasma emission give an access to the gas-phase reactions for the formation of C2 and CN radicals, revealing that C2 radicals are formed mainly in the region near the target while CN radicals can be formed in a much larger region not only in the vicinity of the target, but especially in the region near a substrate far away from the target. [ABSTRACT FROM AUTHOR]