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Understanding how the orbital motion of electrons is coupled to the spin degree of freedom in nanoscale systems is central for applications in spin-based electronics and quantum computation. Here we demonstrate such spin-orbit coupling in a carbon-nanotube quantum dot in the general multielectron regime and in the presence of finite disorder. Also, we find a systematic dependence of the spin-orbit coupling on the electron occupation of the quantum dot. Such a dependence has not been seen in any other system and follows from the curvature-induced spin-orbit-split Dirac spectrum of the underlying graphene lattice. Our findings suggest that the spin-orbit coupling is a general property of carbon-nanotube quantum dots, which should provide a unique platform for the study of spin-orbit effects and their applications. [ABSTRACT FROM AUTHOR]

Presents research which reported a transition from ionic to covalent bonding in a quantum-dot artificial molecule probed by microwave excitations. What quantum dots are; Connecting such dots to current and voltage contacts; Effects of the strength of inter-dot coupling; Demonstration of controllable quantum coherence; Practical applications of research.

We investigate background charge fluctuation in a GaAs quantum dot device by measuring 1/f noise in the single-electron tunneling current through the dot. The current noise is understood as fluctuations of the confinement potential and tunneling barriers. The estimated potential fluctuation increases almost linearly with temperature, which is consistent with a simple model of the 1/f noise. We find that the fluctuation increases very slightly when electrons are injected into excited states of the quantum dot. [ABSTRACT FROM AUTHOR]

Single-electron tunneling through a quantum dot is detected by means of a radio-frequency single-electron transistor. Poisson statistics of single-electron tunneling events are observed from frequency domain measurements, and individual tunneling events are detected in the time-domain measurements. Counting tunneling events gives an accurate current measurement in the saturated current regime, where electrons tunnel into the dot only from one electrode and tunnel out of the dot only to the other electrode. © 2004 American Institute of Physics. [ABSTRACT FROM AUTHOR]

We have experimentally identified the exchange-induced spin blockade in a GaAs double quantum dot. The transport is suppressed only when the eigenstates are well-defined singlet and triplet states, and thus sensitive to dynamic nuclear-spin polarization that causes singlet-triplet mixing. This gives rise to unusual current spectra, such as a sharp current dip and an asymmetric current profile near the triplet resonance of a double quantum dot. Numerical simulations suggest that the current dip is a signature of identical nuclear-spin polarization in the two dots, which is attractive for coherent spin manipulations in a material with nuclear spins. [ABSTRACT FROM AUTHOR]

The tunneling rates for spin-up and -down electrons are investigated for a GaAs quantum dot in an in-plane magnetic field by using a real-time single-electron counting scheme with a nearby charge detector. An extremely small spin-polarized current on the order of attoamperes is analyzed with the spin and energy dependences of the tunneling rates. Fully spin-polarized current is obtained when only a spin-up Zeeman sublevel is located in the transport window. When both Zeeman sublevels are allowed to contribute to the transport, we find that the tunneling rate for spin-up electrons is considerably higher than that for spin-down electrons. This partially spin-polarized current can be explained by the exchange-enhanced spin splitting in low-density regions near the tunneling barriers. [ABSTRACT FROM AUTHOR]

By means of sequential and cotunneling spectroscopy, we study the tunnel couplings between metallic leads and individual levels in a carbon nanotube quantum dot. The levels are ordered in shells consisting of two doublets with strong- and weak-tunnel couplings, leading to gate-dependent level renormalization. By comparison to a one- and two-shell model, this is shown to be a consequence of disorder-induced valley mixing in the nanotube. Moreover, a parallel magnetic field is shown to reduce this mixing and thus suppress the effects of tunnel renormalization. [ABSTRACT FROM AUTHOR]

We investigate how the orbital magnetic moments of electron and hole states in a carbon nanotube quantum dot depend on the number of carriers on the dot. Low temperature transport measurements are carried out in a setup where the device can be rotated in an applied magnetic field, thus enabling accurate alignment with the nanotube axis. The field dependence of the level structure is measured by excited state spectroscopy and excellent correspondence with a single-particle calculation is found. In agreement with band structure calculations we find a decrease of the orbital magnetic moment with increasing electron or hole occupation of the dot, with a scale given by the band gap of the nanotube. [ABSTRACT FROM AUTHOR]

We use a photon-assisted tunneling (PAT) technique to study the high-frequency response of one- and two-electron states in a semiconductor vertically coupled double-dot system. In particular, PAT associated with two-electron spin states in the spin-blockade regime is observed up to the absorption of 10 photons, indicating the preservation of long relaxation times and hence the robustness of our electron spin device under strong microwave irradiation. An alternative double-dot structure with greater flexibility in tuning the inter-dot coupling is presented and its transport characteristics are discussed. This structure is proposed for high-frequency control of two-electron spin states, as required for quantum computation schemes using electron spins in quantum dots. [Copyright &y& Elsevier]