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In order to clearly understand the physical images of incident ions passing through the insulating nanocapillary, in this work we establish a theoretical model, in which the matlab program is combined with the Monte Carlo method, to estimate the time evolution of transmission features, such as the angular and deposited charge distribution, three-dimensional (3D) trajectories of H+ particles with proton incident energies of 10 keV, 100 keV and 1 MeV at -1 title angle. The simulation results show that the transmission mechanism of 100 keV protons is different from those of 10 keV and 1 MeV protons. After a sufficiently charging and discharging stage, 10 keV H+ particles are guided along the direction of capillary axis, indicating that the guiding force from the surface charge patches is significant, and the small-angle scattering of 1 MeV protons under the capillary inner wall is a physical process that determines the transport of H+ particles through the nanocapillary. However, for 100 keV H+ particles, the centroid angle gradually shifts from the guiding direction to the direction close to the incident beam, which is attributed to the fact that the stochastic inelastic binary collision below the surface is the main transmission mechanism at the beginning. After the charging and discharging reach an equilibrium state, the H+ particles are likely to pass through the nanocapillary, and the main transmission mechanism is the charge-patch-assisted specular scattering. This mechanism deepens the understanding of the transport behavior of protons through the nanocapillary, which will contribute to the control and application of the 100 keV proton beam.

The transmissions of oxygen ions through Al2O3 nanocapillaries each 50 nm in diameter and 10 μm in length at a series of different tilt angles are measured, where the ions with energies ranging from 10 to 60 keV and charge states from 1 up to 6 are involved. The angular distribution and the transmission yields of transported ions are investigated. Our results indicate both the existence of a guiding effect when ions pass through the capillary and a significant dependence of the ion transmission on the energy and the charge state of the ions. The guiding effects are observed to be enhanced at lower projectile energies and higher charge states. Meanwhile, the results also exhibit that the transmission yields increase as the tilt angle decreases at a given energy and charge state.

This paper reports that the K x-ray spectra of the thin target (47)Ag, (48)Cd, (49)In and (50)Sn were measured by an HPGe semi-conductor detector in collisions with 84.5 MeV (6)C(4+) ions. Our experiment revealed the K alpha x-ray energy shifts were not obvious and the K beta(1) x-ray energy shifts were about 90 similar to 110 eV. The simple model of Burch et al has been previously used to calculate the K x-ray energy shifts due to an additional vacancy in 2p orbit. The present work extends the model of Burch to calculate the x-ray energy shifts of multiple ionized atoms induced by heavy ions with kinetic energy of MeV/u. In addition to our experimental results, many other experimental results are compared with the calculated values by using the model.

This paper reports that at a newly constructed small-angle x-ray scattering station of Beijing Synchrotron Radiation Facility, the topological shape of ligand-free bovine serum albumin in solution has been investigated. An appropriate scattering curve is obtained and the calculated value of the gyration radius is 31.2A±0.25A (1A=0.1 nm) which is coincident with other ones' results. It finds that the low-resolution structure models obtained by making use of ab initio reconstruction methods are fitting the crystal structure of human serum albumin very well. All of these results perform the potential of the beamline to apply to structural biology studies. The characteristics, the defects, and the improving measures of the station in future are also discussed.

The values of direct double-to-single ionization ratio R of helium atoms induced by Cq+, Oq++ (q = 1–4) ions at incident energies from 0.2 to 8.5MeV are measured. Based on the existing model (Shao J X, Chen X M and Ding B W 2007 Phys. Rev. A 75 012701) the effective charge of the projectile is introduced to theoretically estimate the value of R for the partially stripped ions impacting on helium atoms. The results calculated from our 'effective charge' model are in good agreement with the experimental data, and the dependence of the effective charge on the ionization energy of the projectile is also discussed qualitatively.

This paper reports that the ratios of double to single electron loss cross-section (R) of O2+ in collision with Ar and He at the velocity of 1–4ν0 (ν0 is the Bohr velocity) have been obtained by the coincidence technique. The trend of R – V in the experiment indicates that the effective charge varies with injected velocity. The effective charge can be obtained by the n-body classical trajectory Monte Carlo method, which is interpreted by the molecular Coulomb over barrier model.

The L-shell x-ray yields of Zr and Mo bombarded by slow Ar16+ions are measured. The energy of the Ar16+ions ranges from about 150 keV to 350 keV. The L-shell x-ray production cross sections of Zr and Mo are extracted from these yields data. The explanation of these experimental results is in the framework of the adiabatic direct-ionization and the binding energy modified BEA approximation. We consider, in the slow asymmetric collisions such as Ar and Mo/Zr, the transient united atoms (UA) are formed during the ion-surface interaction and the direct-ionization is the main mechanism for the inner-shell vacancy production. Generally, the theoretical results are in good agreement with the experimental data.

Using the slow highly charged ions Xe-129(q+) (q = 25, 26, 27; initial kinetic T-0

The ratios of transfer ionization (TI) to single-electron capture (SC) cross sections have been measured for the collisions of partially stripped Cq+ ions (q = 1-4) with He. The collision velocity ranges from 0.7 to 4.4v(0) (v(0) is the Bohr velocity). The projectile-ion and recoil-ion coincidence technique is used to separate the processes of TI and SC. The ratios reach the maximum when the velocity is about 3.7 v(0). This can be explained qualitatively based on the two-step mechanism. The experimental results are also compared with the results calculated using the classical trajectory Monte Carlo (CTMC) method. The CTMC results are in agreement with the experimental data basically. The discrepancies in higher velocity region are interpreted by the effective charge effect.

The relative partial cross sections for 13C6+–Ar collisions at 4.15–11.08 keV/u incident energy are measured. The cross-section ratios σ2E/σSC, σ3E/σSC, σ4E/σSC and σ5E/σSC are approximately the constants of 0.51±0.05, 0.20±0.03, 0.06±0.03 and 0.02±0.01 in this region. The significance of the multi-electron process in highly charged ions (HCIs) with argon collisions is demonstrated (σME/σSC as high as 0.79±0.06). In multi-electron processes, it is shown that transfer ionization is dominant while pure electron capture is weak and negligible. For all reaction channels, the cross-sections are independent of the incident energy in the present energy region, which is in agreement with the static characteristic of classic models, i.e. the molecular Coulomb over-the-barrier model (MCBM), the extended classical over-the-barrier model (ECBM) and the semiempirical scaling laws (SL). The result is compared with these classical models and with our previous work of 13C6+-Ne collisions [Chin. Phys. Lett. 23 (2006) 95].

The cross-section ratios of double-, triple-, quadruple-, and the total multi-electron processes to the single electron capture process (σDE/σSC, σTE/σSC, σQE/σSC and σME/σSC) as well as the relative ratios among reaction channels in double-electron active, triple-electron active and quadruple-electron active are measured in 13C6+–Ne collision in the energy region of 4.15–11.08 keV/u by employing position-sensitive and time-of-flight coincident techniques. It is determined that the cross-section ratios σDE/σSC, σTE/σSC, σQE/σSC and σME/σSC are approximately the constants of 0.20±0.03, 0.16±0.04, 0.06±0.02 and 0.42±0.05. These values are obviously smaller than the predictions of the molecular Coulomb over-the-barrier model (MCBM) [J. Phys. B 23 (1990) 4293], the extended classical over-the-barrier model (ECBM) [J. Phys. B 19 (1986) 2925] and the semiempirical scaling laws (SL) [Phys. Rev. A 54 (1996) 4127]. However, the relative ratios among partial processes of DE, TE and QE are found to depend on collision energy, which suggests that the collision dynamics depends on the collision velocity. The limitation of velocity-independent character of ECBM, MCBM and SL is undoubtedly shown.

In recent years, by using the etching techniques with great precision, the ion tracks in materials were converted into insulator and metal nanocapillaries. The physical and chemical properties of the inner surface on micro and nano-scales of these capillaries can be investigated by the interaction of ions with the surfaces. Stolterfoht et al. (2002 Phys. Rev. Lett. 88 133201) have found the evidence for capillary guiding in studying the transmission of 3 keV Ne7+ ions (energy/charge E/q approximate to 10(0) kV) through the polymer nanocapillaries. The self-organized charge-up process was thought to inhibit close contact between the ions and the inner capillary walls. Skog et al. (2008 Phys. Rev. Lett. 101 223202) investigated the guiding effect of 7 keV Ne7+ ions (E/q approximate to 10(0) kV) transmitted through SiO2 nanocapillaries, and found the evidence of sequentially formed charge patches along the capillary. For these keV highly charged ions with E/q approximate to 10(0) kV, the charge patches were formed in a very short time, and then the repulsive electric field rapidly becomes strong enough to deflect the ions, then the ions move along the capillary axis without charge exchange. Zhou et al. (2016 Acta Phys. Sin. 65 103401) have investigated the transmission of 100 keV protons (E/q approximate to 10(2) kV) through the nanocapillaries in polycarbonate (PC) membrane. It was found that the transmitted ions are located around the direction of the incident beam, rather than along the capillary axis. This indicated that the transmission mechanism of hundreds of keV protons through nanocapillaries is significantly different from that for keV highly charged ions. For 100 keV protons, several charge patches suppress the protons to penetrate into the surface, and the protons are transmitted via twice specular scattering near the surface and finally emitted along the incident direction. However, the study of the transmission of E/q approximate to 10(1) kV ions through nanocapillaries is still lacking. In this work, we measure the time evolution of the relative transmission rate, charge state and angular distribution as well as the full width at half maximum of 20 keV protons (E/q approximate to 10(1) kV) transmitted through the nanocapillaries in PC membrane at a tilt angle of +1 degrees. We observe a very long time pre-guiding period before the stable guiding process is established. During the pre-guiding period the direction of the transmitted H+ ions changes to the direction of capillary axis gradually. The transmitted H-0 particles are composed of two peaks: the higher and sharper one is nearly in the beam direction, the wider and lower one is around the guiding direction. With the continuous charging-up process, the intensities of the narrow and sharp peak of transmitted H-0 near the beam direction will decrease and disappear at the end. The data indicate that the scattering and guiding forces are both important for E/q approximate to 10(1) kV ions during the period of pre-guiding process, and the guiding force is dominant till a long time pre-guiding period is ended. This finding will fill in the gap between E/q approximate to 10(0) kV and 10(2) kV of previous studies of ions transmitted through nanocapillaries. It is also helpful for finding the applications of nano-and micro-sized ion beams produced by tapered glass capillary with E/q approximate to 10(1) kV.

The transmission of 1.5 keV-electrons through a conical glass capillary is reported. This study aims to understand the so-called guiding effect for the negatively charged particles (e.g. electrons). The guiding mechanism is understood quite well with positively charged particles in particular highly charged ions, but not clear with electrons, i.e., even the basic scheme mediated by the existence of negative charge patches to guide the electrons is still somewhat controversial. The study of the charging-up dynamics causing the electrons transport inside the capillary will shed light on this issue. In order to perform this, a data acquisition system has been setup to follow the time evolution of the twodimensional angular distribution of the transmitted electrons. The electrons are detected by the multi-channel plate (MCP) detector with a phosphor screen. The image from the phosphor screen is recorded by a charge-coupled device camera. The timing signals for the detected events are extracted from the back stack of the MCP detector and recorded by the data acquisition system, synchronized with the acquired images. The electron beam has a size of 0.5 mm0.5 mm and a divergence of less than 0.35. The inner diameter of the straight part of the capillary is 1.2 mm and the exit diameter is 225 m. A small conducting aperture of 0.3 mm in diameter is placed at the entrance of the capillary. Two-dimensional angular distribution of the transmitted electrons through conical glass capillary and its time evolution are measured. The results show that the transmission rate decreases and reaches to a constant value for the completely discharged glass capillary with time going by. The centroid of the angular distribution moves to an asymptotic value while the width remains unchanged. These transmission characteristics are different from those indicated in our previous work (2016 Acta Phys. Sin. 65 204103). The difference originates from the different manipulations of the capillary outer surface. A conducting layer is coated on the outer surface of the capillary and grounded in this work. This isolates various discharge/charge channels and forms a new stable discharge channel. The transmission rate as a function of the tilt angle shows that the allowed transmission occurs at the tilt angle limited by the geometrical factors, i.e., the geometrical opening angle given by the aspect ratio as well as the beam divergence. The transmission characteristics suggest that most likely there are formed no negative patches to facilitate the electron transmission through the glass capillary at this selected beam energy. It is different from that of highly charged ions, where the formation of the charge patches prohibits the close collisions between the following ions and guides them out of the capillary.

Graphene was first discovered in 2004 (Novoselov K S, et al. 2004 Science 306 666), it is a single atomic layer of sp2-bonded carbon atoms arranged in a honeycomb-like lattice. According to its extraordinary electronic, mechanical, thermal and optical properties, one can expect it to have a variety of applications in nanoscale electronics, composite materials, energy storage, and biomedicine fields. Although many experimental and theoretical studies on graphene have been carried, there still exist many obstacles to its applications. A representative example is nanoscale electronics (e.g., field-effect transistors and optoelectronic devices) that requires non-zero band-gap. Therefore, introducing defects into graphene and leading to band-gap opening are key steps for its technique applications.Recently, ion beam irradiation as a defects introducing technique was performed by Lee et al. (2015 Appl. Surf. Sci. 344 52) and Zeng et al. (2016 Carbon 100 16) through 5, 10, and 15 MeV protons and highly charged ions (HCIs) irradiating the graphene separately. Considering the advantages of simplity for preparing samples and feasibility in atmospheric condition of Raman spectroscopy compared with common characterization techniques (high resolution transmission electron microscopy, scanning electron microscopy, atomic force microscopy) for nano-materials, in both studies, Raman spectroscopy is used to obtain the evolution of ID/IG (ID is the peak intensity excited by defects, IG is the peak intensity origining from lateral vibration of carbon atoms) with different energies and fluences, respectively. In this work, considered are the following points:1) the absence of quantitive characterization for defects in the above two studies; 2) the low displacement energy of 25 eV required for a carbon atom to be knocked out (Zhao S J, et al. 2012 Nanotechnology 23 285703); 3) the complex interaction between HCIs and material. The irradiation effects of single layer graphene on silicon substrate are investigated by 750 keV and 1 MeV proton bombarding. This introduces the defects into graphene and thus leads to band-gap opening. By comparing Raman spectra of the samples before and after irradiation, a quantitive characterization about defects in graphene is achieved. Detailed analysis shows that 1) the value of ID/IG increases with the energy loss of incident proton, which is consistent with the result of SRIM simulation; 2) the average distance of defects LD increases with the incident proton energy; 3) the defect density nD decreases with the incident proton energy. These indicate that the damage effect for MeV protons in single layer graphene with substrate is similar to those in three-dimensional materials. The method presented here may facilitate the understanding of the physical mechanism of MeV proton interaction with two-dimensional materials, and provide a potential way of controlling the electronic structure and band-gap.

In this paper we report the measurements of the K x-ray relative transition probabilities as follows: K-beta/K-alpha for the atomic numbers Z = 39, 51, 62, 63, 64, 66, 67 and 68; and K-alpha2/k(alpha1), k(beta1)(1)/k(alpha1), k(beta2)(1)/k(beta1)1, and k(beta3)/k(beta2) for the atomic numbers Z = 62, 63, 64, 66, 67 and 68 as induced by protons at an energy of 3 MeV. The experimental results obtained are then compared with relativistic Hartree-Fock calculations.

We investigate angular distributions of the transmitted 60 keV and 120 keV O3+ ions through nanocapillaries with 50nm diameter and 10μm length. The experimental results are in agreement with the 'guiding effect' found by Stolterfoht et al. For different tilted angles of the nanocapillary membrane with respect to the beam, the angular distributions of the transmitted ions are measured by a one-dimensional micro-channel plate (MCP) detector. Moreover, the dependence of this guiding effect on the projectile energy is studied.

The Cu films are deposited on two kinds of p-type Si (111) substrates by ionized cluster beam (ICB) technique. The interface reaction and atomic diffusion of Cu/Si (111) and Cu/SiO2/Si (111) systems are studied at different annealing temperatures by x-ray diffraction (XRD) and Rutherford backscattering spectrometry (RBS). Some significant results are obtained: For the Cu/Si (111) samples prepared by neutral clusters, the interdiffusion of Cu and Si atoms occurs when annealed at 230?C. The diffusion coefficients of the samples annealed at 230?C and 500?C are 8.5 ? 10-15 cm2?s-1 and 3.0 ? 10-14 cm2?s-1, respectively. The formation of the copper-silicide phase is observed by XRD, and its intensity becomes stronger with the increase of annealing temperature. For the Cu/SiO2/Si (111) samples prepared by neutral clusters, the interdiffusion of Cu and Si atoms occurs and copper silicides are formed when annealed at 450?C. The diffusion coefficients of Cu in Si are calculated to be 6.0 ? 10-16 cm2?s-1 at 450?C, due to the fact that the existence of the SiO2 layer suppresses the interdiffusion of Cu and Si.

A simple model for the direct ionization and transfer ionization probabilities in A2+ +He collisions in a wide projectile energy range is proposed based on the Bohr–Lindhard model and the classical statistical model. The calculated cross sections are in satisfactory agreement with the experimental data available.

The multi-electron processes are investigated for 17.9–120 keV/u C1+, 30–323 keV/u C2+, 120–438 keV/u C3+, 287–480 keV/u C4+ incident on a helium target. The cross-section ratios of double electron (DE) process to the total of the single electron (SE) and the double electron process (i.e. SE+DE), the direct double electron (DDI) to the direct single ionization (DSI) as well as the contributions of DDI to DE and of TI to DE are measured using coincidence techniques. The energy and charge state dependences of the measured cross-section ratios are studied and discussed.

The cross section ratios of the double, triple and quadruplicate ionization to the single ionization of argon by 1.5-7.5 MeV partially stripped carbon ions are measured by using time-of-flight technique. The Auger transition and the charge exchange process in the multiple ionization of argon are studied. The ratios of cross sections of the direct multiple ionization to those of the direct single ionization are obtained by subtracting the parts of the Auger transition and the charge exchange process from the measured data. It is found that the cross section ratios of the direct multiple ionization to those of the direct single ionization are in good agreement with the predicted multi-step (ν/qeff)-2n+2 law.

The isotopic bare ion 13C6+ was employed to collide with helium at 4.15–11.08 keV/u. The relative partial cross sections were measured by position-sensitive and time-of-flight coincident techniques. It is shown that the direct-ionization (DI) process can be completely ignored in this region, the transfer ionization (TI) process is the most important double-electron channel, and the probability of the pure double-electron capture (DC) process is quite small. The cross-section ratio of the total double-electron (DE) process (i.e. DC+TI) to the single-electron capture (SC) process is experimentally determined to be approximately a constant of 0.09±0.03 in this region, and this value is obviously smaller than the predictions of the classical over-barrier models and the semi-empirical scaling laws. It is found that the cross-section ratio of pure DC to DE decreases obviously as the projectile velocity increases. Because the pure DC process only comes from the radiation de-excitation following the DC process and are competed by the TI process (comes from the auto-ionization following the DC process), this implies that the population of the two captured electrons depends distinctly on the collision velocity. Comparison with works on Ar16+–He by Wu et al. [Phys. Rev. A 48 (1993) 3617] reveals that the strong projectile-dependent character of the pure DC process exists.

We study the L x-ray emission from Zr, Mo and In targets and M x-ray emission from Pb target under bombardment of low energy Arq+ (q = 13,14,15,16) ions. The relative x-ray yields were measured in the projectile kinetic energy range 210–360 keV. It is found that the relative x-ray yields from Zr, Mo and Pb targets increase with the increasing projectile kinetic energy for Ar14+ and Ar16+ projectiles and depend on the potential energy of the projectile remarkably.

When a lambda hyperon was embedded in a nucleus, it can form a hypernucleus. The lifetime and its mass dependence of stable hypernuclei provide information about the weak decay of lambda hyperon inside nuclear medium. This work will introduce the Jefferson Lab experiment (E02-017) which aims to study the lifetime of the heavy hypernuclei using a specially developed fission fragment detection technique, a multi-wire proportional chamber operated under low gas pressure (LPMWPC). Presented here are the method and performance of the reconstruction of fission position on the target foil, the separation of target materials at different regions and the comparison and verification with the Mote Carlo simulation., Comment: 10 pages