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Dynamic critical fluctuations in magnetic materials encode important information about magnetic ordering in the associated critical exponents. Using nitrogen-vacancy centers in diamond, we implement $T_2$ (spin-decoherence) noise magnetometry to study critical dynamics in a 2D Van der Waals magnet CrSBr. By analyzing NV decoherence on time scales approaching the characteristic correlation time $\tau_c$ of critical fluctuations, we extract the critical exponent $\nu$ for the correlation length. Our result deviates from the Ising prediction and highlights the role of long-range dipolar interactions in 2D CrSBr. Furthermore, analyzing the divergence of the correlation length suggests the possibility of 2D-XY criticality in CrSBr in a temperature window near $T_C$ where static magnetic domains are absent. Our work provides a first demonstration of $T_2$ noise magnetometry to quantitatively analyze critical scaling behavior in 2D materials., Comment: 19 pages main text, 4 main text figures, 26 pages Supplementary Materials, 13 Supplementary figures

The excited orbitals of color centers typically show stronger electric dipoles, which can serve as a resource for entanglement, emission tuning, or electric field sensing. Here, we use resonant laser excitation to expose strong transition dipoles in the excited state (ES) orbitals of the negatively charged nitrogen vacancy center in diamond. By applying microwave electric fields, we perform strong Rabi driving between ES orbitals, and show that the dressed states can be tuned in frequency and are protected against fluctuations of the transverse electric field. In contrast with previous results, we observe sharp microwave resonances between magnetic states of the ES orbitals, and find that they are broadened due to simultaneous electric dipole driving.

Color centers in wide-bandgap semiconductors feature metastable charge states that can be interconverted with the help of optical excitation at select wavelengths. The distinct fluorescence and spin properties in each of these states have been exploited to show storage of classical information in three dimensions, but the memory capacity of these platforms has been thus far limited by optical diffraction. Here, we leverage local heterogeneity in the optical transitions of color centers in diamond to demonstrate selective charge state control of individual point defects sharing the same diffraction-limited volume. Further, we apply this approach to dense color center ensembles, and show rewritable, multiplexed data storage with large areal density. These results portend alternative approaches to information processing in the form of devices with enhanced optical storage capacity.

The last decade has seen an explosive growth in the use of color centers for metrology applications, the paradigm example arguably being the nitrogen-vacancy (NV) center in diamond. Here, we focus on the regime of cryogenic temperatures and examine the impact of spin-selective, narrow-band laser excitation on NV readout. Specifically, we demonstrate a more than four-fold improvement in sensitivity compared to that possible with non-resonant (green) illumination, largely due to a boost in readout contrast and integrated photon count. We also leverage nuclear spin relaxation under resonant excitation to polarize the 14N host, which we then prove beneficial for spin magnetometry. These results open opportunities in the application of NV sensing to the investigation of condensed matter systems, particularly those exhibiting superconducting, magnetic, or topological phases selectively present at low temperatures.

Recent advancements with trapped nano- and micro-particles have enabled the exploration of motional states on unprecedented scales. Rotational degrees of freedom stand out due to their intrinsic non-linearity and their coupling with internal spin degrees of freedom, opening up possibilities for gyroscopy and magnetometry applications and the creation of macroscopic quantum superpositions. However, current techniques for fast and reliable rotation of particles with internal spins face challenges, such as optical absorption and heating issues. Here, to address this gap, we demonstrate electrically driven rotation of micro-particles levitating in Paul traps. We show that micro-particles can be set to rotate stably at 150,000 rpm by operating in a hitherto unexplored parametrically driven regime using the particle electric quadrupolar moment. Moreover, the spin states of nitrogen-vacancy centers in diamonds undergoing full rotation were successfully controlled, allowing accurate angular trajectory reconstruction and demonstrating high rotational stability over extended periods. These achievements mark progress toward interfacing full rotation with internal magnetic degrees of freedom in micron-scale objects. In particular, it extends significantly the type of particles that can be rotated, such as ferromagnets, which offers direct implications for the study of large gyromagnetic effects at the micro-scale.

A broad effort is underway to understand and harness the interaction between superconductors and spin-active color centers with an eye on the realization of hybrid quantum devices and novel imaging modalities of superconducting materials. Most work, however, overlooks the complex interplay between either system and the environment created by the color center host. Here we use an all-diamond scanning probe to investigate the spin dynamics of a single nitrogen-vacancy (NV) center proximal to a high-critical-temperature superconducting film in the presence of a weak magnetic field. We find that the presence of the superconductor increases the NV spin coherence lifetime, a phenomenon we tentatively rationalize as a change in the electric noise due to a superconductor-induced redistribution of charge carriers near the NV site. We build on these findings to demonstrate transverse-relaxation-time-weighted imaging of the superconductor film. These results shed light on the complex surface dynamics governing the spin coherence of shallow NVs while simultaneously paving the route to new forms of noise spectroscopy and imaging of superconductors.

We report observations of the Electron Spin Resonance (ESR) of Nitrogen Vacancy (NV) centers in diamonds that are levitating in an ion trap. Using a needle Paul trap operating under ambient conditions, we demonstrate efficient microwave driving of the electronic spin and show that the spin properties of deposited diamond particles measured by the ESR are retained in the Paul trap. We also exploit the ESR signal to monitor the rotation of levitating monocrystals, a first step towards spin-controlled mechanical systems in scattering-free traps., Comment: 6 figures, 8 pages

We report a teleportation experiment involving narrowband entangled photons at 1560 nm and qubit photons at 795 nm emulated by faint laser pulses. A nonlinear difference frequency generation stage converts the 795 nm photons to 1560 nm in order to enable interference with one photon out of the pairs, i.e., at the same wavelength. The spectral bandwidth of all involved photons is of about 25 MHz, which is close to the emission bandwidth of emissive quantum memory devices, notably those based on ensembles of cold atoms and rare earth ions. This opens the route towards the realization of hybrid quantum nodes, i.e., combining quantum memories and entanglement-based quantum relays exploiting either a synchronized (pulsed) or asynchronous (continuous- wave) scenario.