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Co-based honeycomb magnets have been actively studied recently for the potential realization of emergent quantum magnetism therein such as the Kitaev spin liquid. Here we employ density functional and dynamical mean-field theory methods to examine a family of the Kitaev magnet candidates BaCo$_2$($X$O$_4$)$_2$ ($X$ = P, As, Sb), where the compound with $X$ = Sb being not synthesized yet. Our study confirms the formation of Mott insulating phase and the $J_{\rm eff}$ = 1/2 spin moments at Co$^{2+}$ sites despite the presence of a sizable amount of trigonal crystal field in all three compounds. The pnictogen substitution from phosphorus to antimony significantly changes the in-plane lattice parameters and direct overlap integral between the neighboring Co ions, leading to the suppression of the Heisenberg interaction. More interestingly, the marginal antiferromagnetic nearest-neighbor Kitaev term changes sign into a ferromagnetic one and becomes sizable at the $X$ = Sb limit. Our study suggests that the pnictogen substitution can be a viable route to continuously tune magnetic exchange interactions and to promote magnetic frustration for the realization of potential spin liquid phases in BaCo$_2$($X$O$_4$)$_2$., Comment: 8 pages, 4 figures

We employ ab-initio electronic structure calculations to investigate the charge-density waves and periodic lattice distortions in bilayer 2H-NbSe$_2$. We demonstrate that the vertical stacking can give rise to a variety of patterns that may lower the symmetry of the CDW exhibited separately by the two composing 1H-NbSe$_2$ monolayers. The general tendency to a spontaneous symmetry breaking observed in the ground state and the first excited states is shown to originate from a non-negligible inter-layer coupling. Simulated images for scanning tunnelling microscopy (STM) as well as diffraction/scattering patterns show signatures of the different stacking orders. This may not only be useful to reinterpret past experiments on surfaces and thin films, but may also be exploited to devise ad-hoc experiments for the investigation of the stacking order in 2H-NbSe$_2$. We anticipate that our analysis does not only apply to the 2H-NbSe$_2$ bilayer, but is also relevant for thin films and bulk, whose smallest centro-symmetric component is indeed the bilayer. Finally, our results illustrate clearly that the vertical stacking is not only important for 1T structures, as exemplified by the metal-to-insulator transition observed in 1T-TaS$_2$, but seems to be a general feature of metallic layered transition metal dichalcogenides as well., Comment: 11 pages, 5 figures

Metal thin films on soft polymers provide a unique opportunity for resistance-based strain sensors. A mechanical mismatch between the conductive film and the flexible substrate causes cracks to open and close, changing the electrical resistance as a function of strain. However, the very randomness of the formation, shape, length, orientation, and distance between adjacent cracks limits the sensing range as well as repeatability. Herein, we present a breakthrough: the Zerogap Strain Sensor, whereby lithography eliminates randomness and violent tearing process inherent in conventional crack sensors and allows for short periodicity between gaps with gentle sidewall contacts, critical in high strain sensing enabling operation over an unprecedently wide range. Our sensor achieves a gauge factor of over 15,000 at {\epsilon}ext=18%, the highest known value. With the uniform gaps of three-to-ten thousand nanometer widths characterized by periodicity and strain, this approach has far reaching implications for future strain sensors whose range is limited only by that of the flexible substrate, with non-violent operations that always remain below the tensile limit of the metal.

We consider the interplay of the muon $g-2$ anomaly and the proton decay in the SUSY SU(5) GUTs with generation-independent scalar soft masses. In these scenarios, we introduce a number of $\bf 5+{\bar 5}$ messenger fields with doublet-triplet splitting in general gauge mediation to transmit SUSY breaking to the visible sector by gauge loops. As a result, squarks and sleptons receive generation-independent soft SUSY breaking masses, which are split already at the messenger scale. Taking into account the perturbative unification of gauge couplings as well as the bounds from electroweak precision and vacuum stability bounds, we showed the parameter space in general gauge mediation to explain the muon $g-2$ anomaly with smuon and sneutrino loops while evading the strong bounds on squarks and gluinos from the Large Hadron Collider. We also obtained the dominant Higgsino contributions to the proton decay mode, $p\to K^+{\bar\nu}$, with general generation-independent sparticle masses for squarks and sleptons. Even for split scalar soft masses in our model, however, we found that the bounds from the proton decay are satisfied only if the effective Yukawa couplings of the colored Higgsinos are suppressed further by a factor of order $10^{-4}-10^{-3}$. We illustrated how such a suppression factor is realized in orbifold GUTs in the extra dimension where the colored Higgsinos in the bulk are not coupled to the matter fields localized at the orbifold fixed points at the leading order., Comment: 35 pages, 8 figures, v2: typos fixed and reference updated, v3: version to appear in Phys. Rev. D

Using first-principles techniques, we study the structural, magnetic and electronic properties of (111)-oriented (LaMnO$_3$)$_{2n}$$\vert$(SrMnO$_3$)$_{n}$ superlattices of varying thickness ($n=2,4,6$). We find that the properties of the thinnest superlattice ($n=2$) are similar to the celebrated half-metallic ferromagnetic alloy La$_{2/3}$Sr$_{1/3}$MnO$_3$, with quenched Jahn-Teller distortions. At intermediate thickness ($n=4$), the $a^{-}a^{-}a^{-}$ tilting pattern transitions to the $a^{-}a^{-}c^{+}$ tilting pattern, driven by the lattice degrees of freedom in the LaMnO$_3$ region. The emergence of the Jahn-Teller modes and the spatial extent needed for their development play a key role in this structural transition. For the largest thickness considered ($n=6$), we unveil an emergent separation of Jahn-Teller and volume-breathing orders in the ground-state structure with the $a^{-}a^{-}c^{+}$ tilting pattern, whereas it vanishes in the antiferromagnetic configurations. The ground state of all superlattices is half-metallic ferromagnetic, not affected by the underlying series of structural transitions. Overall, these results outline a thickness-induced crossover between the physical properties of bulk La$_{2/3}$Sr$_{1/3}$MnO$_3$ and bulk LaMnO$_3$., Comment: 7 pages excluding references, 8 figures

Nanoconfined waters have been extensively studied within various systems, demonstrating low permittivity under static conditions; however, their dynamics have been largely unexplored due to the lack of a robust platform, particularly in the terahertz (THz) regime where hydrogen bond dynamics occur. We report the THz complex refractive index of nanoconfined water within metal gaps ranging in width from 2 to 20 nanometers, spanning mostly interfacial waters all the way to quasi-bulk waters. These loop nanogaps, encasing water molecules, sharply enhance light-matter interactions, enabling precise measurements of refractive index, both real and imaginary parts, of nanometer-thick layers of water. Under extreme confinement, the suppressed dynamics of the long-range correlation of hydrogen bond networks corresponding to the THz frequency regime result in a significant reduction in the terahertz permittivity of even 'non-interfacial' water. This platform provides valuable insights into the long-range collective dynamics of water molecules which is crucial to understanding water-mediated processes such as protein folding, lipid rafts, and molecular recognition.

The size of the optics used in observatories is often limited by fabrication, metrology, and handling technology, but having a large primary mirror provides significant benefits for scientific research. The evolution of rocket launch options enables heavy payload carrying on orbit and outstretching the telescope's form-factor choices. Moreover, cost per launch is lower than the traditional flight method, which is obviously advantageous for various novel space observatory concepts. The University of Arizona has successfully fabricated many large-scale primary optics for ground-based observatories including the Large Binocular Telescope (LBT, 8.4 meter diameter two primary mirrors), Large Synoptic Survey Telescope (now renamed to Vera C. Rubin Observatory, 8.4 meter diameter monolithic primary and tertiary mirror), and the Giant Magellan Telescope (GMT, 8.4 meter diameter primary mirror seven segments). Launching a monolithic primary mirror into space could bypass many of the difficulties encountered during the assembly and deployment of the segmented primary mirrors. However, it might bring up unprecedented challenges and hurdles, also. We explore and foresee the expected challenges and evaluate them. To estimate the tolerance and optical error budget of a large optical system in space such as three mirror anastigmat telescope, we have developed a methodology that considers various errors from design, fabrication, assembly, and environmental factors., Comment: 6 pages, presented August 2023 at SPIE Optics+Photonics, San Diego, CA, USA

Recent studies have explored the deployment of privacy-preserving deep neural networks utilizing homomorphic encryption (HE), especially for private inference (PI). Many works have attempted the approximation-aware training (AAT) approach in PI, changing the activation functions of a model to low-degree polynomials that are easier to compute on HE by allowing model retraining. However, due to constraints in the training environment, it is often necessary to consider post-training approximation (PTA), using the pre-trained parameters of the existing plaintext model without retraining. Existing PTA studies have uniformly approximated the activation function in all layers to a high degree to mitigate accuracy loss from approximation, leading to significant time consumption. This study proposes an optimized layerwise approximation (OLA), a systematic framework that optimizes both accuracy loss and time consumption by using different approximation polynomials for each layer in the PTA scenario. For efficient approximation, we reflect the layerwise impact on the classification accuracy by considering the actual input distribution of each activation function while constructing the optimization problem. Additionally, we provide a dynamic programming technique to solve the optimization problem and achieve the optimized layerwise degrees in polynomial time. As a result, the OLA method reduces inference times for the ResNet-20 model and the ResNet-32 model by 3.02 times and 2.82 times, respectively, compared to prior state-of-the-art implementations employing uniform degree polynomials. Furthermore, we successfully classified CIFAR-10 by replacing the GELU function in the ConvNeXt model with only 3-degree polynomials using the proposed method, without modifying the backbone model.

In this paper, we employ the Physics-Informed Neural Network (PINN) to estimate the practical range of the characteristic wavelength parameter(referred to as the smoothing parameter) $\alpha$ in the Leray-Burgers equation. The Leray-Burgers equation, a regularization of the inviscid Burgers equation, incorporates a Helmholtz filter with a characteristic wavelength $\alpha$ to replace the usual convective velocity, inducing a regularized convective velocity. The filter bends the equation's characteristics slightly and makes them not intersect each other, leading to a global solution in time. By conducting computational experiments with various initial conditions, we determine the practical range of $\alpha >0$ that closely approximates the solutions of the inviscid Burgers equation. Our findings indicate that the value of $\alpha$ depends on the initial data, with the practical range of $\alpha$ being between 0.01 and 0.05 for continuous initial profiles and between 0.01 and 0.03 for discontinuous initial profiles. The Leray-Burgers equation captures shock and rarefaction waves within the temporal domain for which training data exists. However, as the temporal domain extends beyond the training interval, data-driven forward computation demonstrates that the predictions generated by the PINN start to deviate from the exact solutions. This study also highlights the effectiveness and efficiency of the Leray-Burgers equation in real practical problems, specifically Traffic State Estimation.

We consider the relic density and positivity bounds for freeze-in scalar dark matter with general Higgs-portal interactions up to dimension-8 operators. When dimension-4 and dimension-6 Higgs-portal interactions are proportional to mass squares for Higgs or scalar dark matter in certain microscopic models such as massive graviton, radion or general metric couplings with conformal and disformal modes, we can take the dimension-8 derivative Higgs-portal interactions to be dominant for determining the relic density via the 2-to-2 thermal scattering of the Higgs fields after reheating. We discuss the implications of positivity bounds for microscopic models. First, massive graviton or radion mediates attractive forces between Higgs and scalar dark matter and the resultant dimension-8 operators respect the positivity bounds. Second, the disformal couplings in the general metric allow for the subluminal propagation of graviton but violate the positivity bounds. We show that there is a wide parameter space for explaining the correct relic density from the freeze-in mechanism and the positivity bounds can curb out the dimension-8 derivative Higgs-portal interactions nontrivially in the presence of the similar dimension-8 self-interactions for Higgs and dark matter., Comment: 20 pages, 4 figures, v2: expanded discussion on microscopic models and freeze-in contribution from higher dimensional operators. Version to appear in JHEP

Non-fungible tokens (NFTs) are becoming increasingly popular in Play-to-Earn (P2E) Web3 applications as a means of incentivizing user engagement. In Web3, users with NFTs ownership are entitled to monetize them. However, due to lack of objective NFT valuation, which makes NFT value determination challenging, P2E applications ecosystems have experienced inflation. In this paper, we propose a method that enables NFT inflation value management in P2E applications. Our method leverages the contribution-rewards model proposed by Curve Finance and the automated market maker (AMM) of decentralized exchanges. In decentralized systems, P2E Web3 applications inclusive, not all participants contribute in good faith. Therefore, rewards are provided to incentivize contribution. Our mechanism proves that burning NFTs, indicating the permanent removal of NFTs, contributes to managing inflation by reducing the number of NFTs in circulation. As a reward for this contribution, our method mints a compensation (CP) token as an ERC-20 token, which can be exchanged for NFTs once enough tokens have been accumulated. To further increase the value of the CP token, we suggest using governance tokens and CP tokens to create liquidity pools for AMM. The value of the governance token is determined by the market, and the CP token derives its value from the governance token in AMM. The CP token can determine its worth based on the market value of the governance token. Additionally, since CP tokens are used for exchanging NFTs, the value of the NFT is ultimately determined by the value of the CP token. To further illustrate our concept, we show how to adjust burning rewards based on factors such as the probability of upgrading NFTs' rarity or the current swap ratio of governance and CP tokens in AMM.

We present a molecular orbital candidate Ba$_{4}$TaMn$_{3}$O$_{12}$ with a face-sharing octahedra trimer, by comparing it with a related compound Ba$_{4}$NbMn$_{3}$O$_{12}$. The synthesis of the polycrystalline powder is optimized by suppressing the secondary impurity phase via x-ray diffraction. Magnetic susceptibility measurements on the optimized samples reveal a weak magnetic hysteresis with magnetic transitions consistent with heat capacity results. The effective magnetic moments from susceptibility indicate a strongly coupled $S=2$ antiferromagnetic trimer at around room temperature, whereas the estimated magnetic entropy from heat capacity suggests the localized $S=3/2$ timer. These results can be explainable by a partial molecular orbital state, in which three $t_{2g}$ electrons are localized in each Mn ion and one $e_{g}$ electron is delocalized over two-end Mn ions of the trimer based on density functional theory calculations. This unconventional 3$d$ orbital state is comprehended as a consequence of competition between the hybrid interatomic orbitals within the Mn trimer and the local moment formation by on-site Coulomb correlations., Comment: 15 pages, 12 figures, 4 tables

Right feeble groups are defined as groupoids $(X,*)$ such that (i) $x, y\in X$ implies the existence of $a, b \in X$ such that $a*x = y$ and $b*y = x$. Furthermore, (ii) if $x, y, z \in X$ then there is an element $w\in X$ such that $x*(y*z) = w*z$. These groupoids have a "remnant" group structure, which includes many other groupoids. In this paper, we investigate some properties of these groupoids. Enough examples are supplied to support the argument that they form a suitable class for systematic investigation., Comment: submitted

Kagome lattice has been actively studied for the possible realization of frustration-induced two-dimensional flat bands and a number of correlation-induced phases. Currently, the search for kagome systems with a nearly dispersionless flat band close to the Fermi level is ongoing. Here, by combining theoretical and experimental tools, we present Sc$_3$Mn$_3$Al$_7$Si$_5$ as a novel realization of correlation-induced almost-flat bands in the kagome lattice in the vicinity of the Fermi level. Our magnetic susceptibility, $^{27}$Al nuclear magnetic resonance, transport, and optical conductivity measurements provide signatures of a correlated metallic phase with tantalizing ferromagnetic instability. Our dynamical mean-field calculations suggest that such ferromagnetic instability observed originates from the formation of nearly flat dispersions close to the Fermi level, where electron correlations induce strong orbital-selective renormalization and manifestation of the kagome-frustrated bands. In addition, a significant negative magnetoresistance signal is observed, which can be attributed to the suppression of flat-band-induced ferromagnetic fluctuation, which further supports the formation of flat bands in this compound. These findings broaden a new prospect to harness correlated topological phases via multiorbital correlations in 3$d$-based kagome systems., Comment: 14 pages, 7 figures

Future generation technologies demand high efficiency photodetectors to enable sensing and switching devices for ultrafast communication and machine vision. This require direct-band gap materials with high photosensitivity, high detectivity and high quantum efficiency. Monolayered two- Dimensional (2D)-Semiconductors based photodetectors are the most promising materials for such applications, although experimental realization has been limited due to unavailability of high quality sample. In the current manuscript, we report about WS$_2$ based photodetector having sensitivity of 290 AW-1 upon 405 nm excitation and incident power density as low as 0.06 mW/cm$^2$. The fabricated device shows detectivity of 52*10^14 with external quantum efficiency of 89*10$^3$%. The observed superior photo-response parameters of CVD grown WS$_2$ based photodetector as compared to Si-detectors establishes it capability to replace the Si-photodetectors with monolayered ultrathin device having superior performance parameters., Comment: 26 Pages, 8 figures

Many practical applications, ranging from paper-reviewer assignment in peer review to job-applicant matching for hiring, require human decision makers to identify relevant matches by combining their expertise with predictions from machine learning models. In many such model-assisted document matching tasks, the decision makers have stressed the need for assistive information about the model outputs (or the data) to facilitate their decisions. In this paper, we devise a proxy matching task that allows us to evaluate which kinds of assistive information improve decision makers' performance (in terms of accuracy and time). Through a crowdsourced (N=271 participants) study, we find that providing black-box model explanations reduces users' accuracy on the matching task, contrary to the commonly-held belief that they can be helpful by allowing better understanding of the model. On the other hand, custom methods that are designed to closely attend to some task-specific desiderata are found to be effective in improving user performance. Surprisingly, we also find that the users' perceived utility of assistive information is misaligned with their objective utility (measured through their task performance).

We consider the positivity bounds for WIMP scalar dark matter with effective Higgs-portal couplings up to dimension-8 operators. Taking the superposed states for Standard Model Higgs and scalar dark matter, we show that the part of the parameter space for the effective couplings, otherwise unconstrained by phenomenological bounds, is ruled out by the positivity bounds on the dimension-8 derivative operators. We find that dark matter relic density, direct and indirect detection and LHC constraints are complementary to the positivity bounds in constraining the effective Higgs-portal couplings. In the effective theory obtained from massive graviton or radion, there appears a correlation between dimension-8 operators and other effective Higgs-portal couplings for which the strong constraint from direct detection can be evaded. Nailing down the parameter space mainly by relic density, direct detection and positivity bounds, we find that there are observable cosmic ray signals coming from the dark matter annihilations into a pair of Higgs bosons, $WW$ or $ZZ$., Comment: 31 pages, 6 figures, v2: one-loop corrections to the positivity bounds added, version to be published in JHEP

By employing first-principles electronic structure calculations we investigate nickelate superlattices [LaNiO$_3$]$_1$/[LaAlO$_3$]$_1$ and [LaNiO$_3$]$_1$/[SrTiO$_3$]$_1$ with (001) orientation under epitaxial tensile strain. Within density functional theory augmented by mean-field treatement of on-site electronic correlations, the ground states show remarkable dependence on the correlation strength and the strain. In the weakly and intermediately correlated regimes with small epitaxial strain, the charge-disproportionated insulating states with antiferromagneitc order is favored over the other orbital and spin ordered phases. On the other hand, in the strongly correlated regime or under the large tensile strain, ferromagnetic spin states with Jahn-Teller orbital order become most stable. The effect from polar interfaces in LaNiO$_3$]$_1$/[SrTiO$_3$]$_1$ is found to be noticeable in our single-layered geometry. Detailed discussion is presented in comparison with previous experimental and theoretical studies., Comment: 9 pages, 8 figures

Modern societies have adopted government-issued fiat currencies many of which exist today mainly in the form of digits in credit and bank accounts. Fiat currencies are controlled by central banks for economic stimulation and stabilization. Boom-and-bust cycles are created. The volatility of the cycle has become increasingly extreme. Social inequality due to the concentration of wealth is prevalent worldwide. As such, restoring sound money, which provides stored value over time, has become a pressing issue. Currently, cryptocurrencies such as Bitcoin are in their infancy and may someday qualify as sound money. Bitcoin today is considered as a digital asset for storing value. But Bitcoin has problems. The first issue of the current Bitcoin network is its high energy consumption consensus mechanism. The second is the cryptographic primitives which are unsafe against post-quantum (PQ) attacks. We aim to propose Green Bitcoin which addresses both issues. To save energy in consensus mechanism, we introduce a post-quantum secure (self-election) verifiable coin-toss function and novel PQ secure proof-of-computation primitives. It is expected to reduce the rate of energy consumption more than 90 percent of the current Bitcoin network. The elliptic curve cryptography will be replaced with PQ-safe versions. The Green Bitcoin protocol will help Bitcoin evolve into a post-quantum secure network., Comment: 16 pages

In this work, the influence of Au plasmonics on photocurrent generation in the visible wavelength range in integrated thiol-linked CdSe quantum dot/Au nanogap structures is demonstrated. The plasmonic absorption is sensed utilizing photoacoustic (PA) detection technique. The laser diode is modulated to generate the PA excitation that oscillates the air-filled cell. When light absorption increases, an enhanced acoustic signal is captured by a microphone. The observed enhancement in the PA response is related to plasmonic absorption by the Au layers and the response is further enhanced by about 20% due to CdSe QDs. In our structure, the surface plasmon resonance (SPR) wavelength is approximately 500 nm. The SPR is utilized for generating photocurrents in CdSe quantum dots. Due to energy transfer from the dot to closely spaced Au surface through thiol links, a smooth transmission channel of electrons is established that forms a detectable photocurrent, which can be tuned by a bias voltage. These plasmonic nanogap structures can enable higher sensitivity in photovoltaics, photodetection and sensing.

We propose a novel model which extends the Standard Model (SM) by introducing a $SU(2)_D$ gauge symmetry. In this model, a dark $SU(2)_D$ Higgs doublet and a Higgs bi-doublet can contribute to the muon $g-2$ anomaly and the $W$ boson mass, remaining in tune with the recent experimental results. At the same time, the isospin charged gauge boson of $SU(2)_D$ becomes a plausible candidate for Dark Matter(DM). We find that the resulting parameter space can fit the muon $g-2$, the $W$ boson mass and the DM constraints simultaneously., Comment: 6 pages, 2 figures, Proceeding for IDM 2022, 14th International Conference on Identification of Dark Matter, Vienna, Austria

Ethereum and its standardized token interface have formed decentralized finance (DeFi), an open financial system based on blockchain smart contracts. The DeFi ecosystem has become richer with the introduction of DeFi composability projects, such as Lido finance and Curve finance. DeFi composability denotes the concatenation of DeFi services in which each DeFi service locks assets as collateral and gives another asset as liquidity of locked assets to providers. Providers use the tokens given for other concatenated DeFi services, such as lending, decentralized exchanges (DEXs), and derivatives. The DeFi ecosystem uses ERC-20 tokens which can represent the value of an asset. ERC-721 non-fungible tokens (NFTs) are not widely adopted in DeFi, since they represent rights to an asset and are not considered appropriate for valuation. In this paper, we propose a new concept, perpetual contract NFT, which exploits perpetual future contracts in the cryptocurrency derivatives market. Unlike futures contracts in a traditional derivatives market, in the cryptocurrency derivatives market, most futures contracts are perpetual. In addition, the value of futures contract is backed by collateral. Therefore, if we mint the rights to perpetual contracts as NFT, we can use the perpetual contract NFT as collateral for DeFi composability. To validate our proposal and its profitability, we experiment with the position NFT of Uniswap v3. Through validation, we show that our concept works in real-world scenarios.

We report Chern insulating phases emerging from a single layer of layered chalcogenide CrSiTe$_{3}$, a transition metal trichacogenides (TMTC) material, in the presence of charge doping. Due to strong hybridization with Te $p$ orbitals, the spin-orbit coupling effect opens a finite band gap, leading to a nontrivial topology of the Cr $e_{\mathrm{g}}$ conduction band manifold with higher Chern numbers. Our calculations show that quantum anomalous Hall effects can be realized by adding one electron in a formula unit cell of Cr$_{2}$Si$_{2}$Te$_{6}$, equivalent to electron doping by 2.36$\times$10$^{14}$ cm$^{-2}$ carrier density. Furthermore, the doping-induced anomalous Hall conductivity can be controlled by an external magnetic field via spin-orientation-dependent tuning of the spin-orbit coupling. In addition, we find distinct quantum anomalous Hall phases employing tight-binding model analysis, suggesting that CrSiTe$_{3}$ can be a fascinating new platform to realize Chern insulating systems with higher Chern numbers., Comment: 9 pages, 8 figures, and additional supplementary information