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International audience; A β-decay experiment aiming at investigation of the low-spin structure of 100Zr was performed using the GRIFFIN spectrometer at TRIUMFISAC. Based on the obtained data, a new 2 + state is postulated which is degenerate in energy with the established (5+) level at 2209 keV.

The β-delayed one- and two-neutron emission probabilities (P_{1n} and P_{2n}) of 20 neutron-rich nuclei with N≥82 have been measured at the RIBF facility of the RIKEN Nishina Center. P_{1n} of ^{130,131}Ag, ^{133,134}Cd, ^{135,136}In, and ^{138,139}Sn were determined for the first time, and stringent upper limits were placed on P_{2n} for nearly all cases. β-delayed two-neutron emission (β2n) was unambiguously identified in ^{133}Cd and ^{135,136}In, and their P_{2n} were measured. Weak β2n was also detected from ^{137,138}Sn. Our results highlight the effect of the N=82 and Z=50 shell closures on β-delayed neutron emission probability and provide stringent benchmarks for newly developed macroscopic-microscopic and self-consistent global models with the inclusion of a statistical treatment of neutron and γ emission. The impact of our measurements on r-process nucleosynthesis was studied in a neutron star merger scenario. Our P_{1n} and P_{2n} have a direct impact on the odd-even staggering of the final abundance, improving the agreement between calculated and observed Solar System abundances. The odd isotope fraction of Ba in r-process-enhanced (r-II) stars is also better reproduced using our new data.

At the RIKEN Nishina Center, exotic neutron-rich isotopes of Ba, La, Ce, Pr, and Nd were measured. This work reports their half-lives (T1/2) and β-delayed neutron-emission probabilities (Pxn). The setup consisted of the BigRIPS in-flight separator for particle identification, the Advanced Implantation Detector Array (AIDA) for ions and β detection, and the BRIKEN neutron counter for neutron detection. Using this arrangement, 4 new T1/2 and 14 new P1n were measured. Furthermore, 38 T1/2 and 2 P1n values were remeasured, decreasing the uncertainties for some of them. In addition to improving predictions of nucleosynthesis models that describe the production of the rare-earth peak at A ∼ 160 via the r-process, these additional experimental data should help to constrain theoretical models for calculations of T1/2 and Pxn in this region.

An array of 128 CsI(Tl) charged particle detectors providing nearly 4 π coverage has been developed at Simon Fraser University (SFU) and commissioned at TRIUMF, Canada’s particle accelerator center. The new CsI ball array replaces a previous 24-detector array and offers improved charged particle detection efficiency and discrimination between reaction channels due to its increased angular coverage. A technical overview of the CsI ball array, as well as commissioning data including measurements of the charged particle detection efficiency, is presented.

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency γ -ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF’s Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) γ -ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

The β-delayed neutron-emission probabilities of 28 exotic neutron-rich isotopes of Pm, Sm, Eu, and Gd were measured for the first time at RIKEN Nishina Center using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The existing β-decay half-life (T 1/2) database was significantly increased toward more neutron-rich isotopes, and uncertainties for previously measured values were decreased. The new data not only constrain the theoretical predictions of half-lives and β-delayed neutron-emission probabilities, but also allow for probing the mechanisms of formation of the high-mass wing of the rare-earth peak located at A ≈ 160 in the r-process abundance distribution through astrophysical reaction network calculations. An uncertainty quantification of the calculated abundance patterns with the new data shows a reduction of the uncertainty in the rare-earth peak region. The newly introduced variance-based sensitivity analysis method offers valuable insight into the influence of important nuclear physics inputs on the calculated abundance patterns. The analysis has identified the half-lives of 168Sm and of several gadolinium isotopes as some of the key variables among the current experimental data to understand the remaining abundance uncertainty at A = 167–172.

This experiment was performed at RI Beam Factory operated by RIKEN Nishina Center and CNS, University of Tokyo. O.H, T.D, P.J.W, C.G.B, C.J.G and D.K would like to thank STFC, UK for support. This research was sponsored in part by the Office of Nuclear Physics, U.S. Department of Energy under Award No. DE-FG02-96ER40983 (UTK) and DEAC05-00OR22725 (ORNL), and by the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE Award No. DENA0002132. This work was supported by National Science Foundation under Grants No. PHY-1430152 (JINA Center for the Evolution of the Elements), No. PHY-1565546 (NSCL), and No. PHY-1714153 (Central Michigan University). This work was supported by the Polish National Science Center under Contracts No. UMO-2015/18/E/ST2/00217, No. 2017/01/X/ST2/01144, No. 2019/33/N/ST2/03023 and No. 2020/36/T/ST2/00547. This work was also supported by JSPS KAKENHI (Grants No. 14F04808, No. 17H06090, No. 25247045, and No. 19340074). This work was also supported by Spanish Ministerio de Economia y Competitividad grants (FPA2011-06419, FPA2011-28770-C03-03, FPA2014-52823-C2-1-P, FPA2014-52823-C2-2-P, SEV-2014-0398, IJCI-2014-19172), by European Commission FP7/EURATOM Contract No. 605203, by the UK Science and Technology Facilities Council Grant No. ST/N00244X/1, by the National Research Foundation (NRF) in South Korea (No. 2016K1A3A7A09005575, No. 2015H1A2A1030275) and by the Natural Sciences and Engineering Research Council of Canada (NSERC) via the Discovery Grants SAPIN-2014-00028 and RGPAS 462257-2014. TRIUMF receives federal funding via a contribution agreement with the National Research Council Canada. This work was also supported by NKFIH (NN128072), and by the UNKP-20-5-DE-2 New National Excellence Program of the Ministry of Human Capacities of Hungary. G.G.K. acknowledges support from the Janos Bolyai research fellowship of the Hungarian Academy of Sciences. M.W.-C. acknowledges support from the Polish NCN project Miniatura No. 2017/01/X/ST2/01144. Z.L was supported by the National Key Research and Development Program of China (Contract No. 2018YFA0404402), the National Natural Science Foundation of China (Grants No. 11961141004, No. 11735017, No. 11675225 and No. 11635003) and the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB34000000). M.R.M. performed this work under the auspice of the U.S. Department of Energy at Los Alamos National Laboratory. Los Alamos National Laboratory is operated by Triad National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy (Contract No. 89233218CNA000001).

Aquesta es una copia de la versio author’s final draft d'un article publicat a la revista [Physical Review C ]. URL d'aquest document a UPCommons E-prints: http://hdl.handle.net/2117/174873

Lifetimes of ${2}_{1}^{+}$ and ${4}_{1}^{+}$ states as well as some negative-parity and nonyrast states in $^{188--200}\mathrm{Hg}$ were measured using $\ensuremath{\gamma}\ensuremath{-}\ensuremath{\gamma}$ electronic fast timing techniques with the ${\mathrm{LaBr}}_{3}(\mathrm{Ce})$ detector array of the GRIFFIN spectrometer. The excited states were populated in the $\ensuremath{\epsilon}/{\ensuremath{\beta}}^{+}$ decay of ${J}^{\ensuremath{\pi}}={7}^{+}/{2}^{\ensuremath{-}}\phantom{\rule{0.28em}{0ex}}^{188--200}\mathrm{Tl}$ produced at the TRIUMF-ISAC facility. The deduced $B(E2)$ values are compared to different interacting boson model predictions. The precision achieved in this paper over previous ones allows for a meaningful comparison with the different theoretical models of these transitional Hg isotopes, which confirms the onset of state mixing in $^{190}\mathrm{Hg}$.

The elusive $\beta^-\text{p}^+$ decay was observed in $^{11}$Be by directly measuring the emitted protons and their energy distribution for the first time with the prototype Active Target Time Projection Chamber (pAT-TPC) in an experiment performed at ISAC-TRIUMF. The measured $\beta^-\text{p}^+$ branching ratio is orders of magnitude larger than any previous theoretical model predicted. This can be explained by the presence of a narrow resonance in $^{11}$B above the proton separation energy.

The Tz=−32 nucleus 21Mg has been studied by Coulomb excitation on 196Pt and 110Pd targets. A 205.6(1)-keV γ-ray transition resulting from the Coulomb excitation of the 52+ ground state to the first excited 12+ state in 21Mg was observed for the first time. Coulomb excitation cross-section measurements with both targets and a measurement of the half-life of the 12+ state yield an adopted value of B(E2;52+→12+)=13.3(4) W.u. A new excited state at 1672(1) keV with tentative 92+ assignment was also identified in 21Mg. This work demonstrates a large difference in the B(E2;52+→12+) value between T=32, A=21 mirror nuclei. The difference is investigated in the shell-model framework employing both isospin conserving and breaking USD interactions and using modern ab initio nuclear structure calculations, which have recently become applicable in the sd shell. (Less)

© 2019, Springer Nature Switzerland AG. We made an experiment to measure half-lives T1/2 and neutron emission probabilities Pxn of nuclei around mass 80, aiming to improve r-process abundance calculations around the first abundance peak with a new dedicated experimental setup at RIKEN. Details of the experiment and a few preliminary results are presented.

International audience; The evaluated data are presented for 11 known A=218 nulcides (Pb, Bi, Po, At, Rn, Fr, Ra, Ac, Th, Pa and U). For 218 Pb, 218 Bi, 218 At and 218 Pa, data are available only for the ground states. For 218 U, only the g.s. and a high-spin isomer are known, with no data on γ -ray transitions available. For 218 Po, ten excited states are known from 218 Bi decay, with no knowledge on the multipolarities of gamma-ray transitions. For 218 Th, five excited states in the g.s. band are known from an in-beam γ -ray study. Data on level half-lives, multipolarities and mixing ratios of gamma transitions is generally lacking for A=218 nuclei. The static magnetic dipole moment has been measured for only an isomer in 218 Fr. With the exception of a new nuclide, 218 Pb, and measurements of half-lives of ground states of a few nuclides of A=218 and A=222, no substantial structure information has become available since the previous evaluation in 2006. Q values are adopted from 2017Wa10 (AME-2016). The present evaluation supersedes the previous A=218 ENSDF evaluations, 2006Ja03, 1995El08, 1987El12 and 1977To13. This evaluation was carried out as part of a joint IAEA-ICTP workshop for Nuclear Structure and Decay Data, organized and hosted by the IAEA, Vienna, and ICTP, Trieste, October 15–26, 2018.

The SPectrometer for Internal Conversion Electrons (SPICE) has been commissioned for use in conjunction with the TIGRESS $\gamma$-ray spectrometer at TRIUMF's ISAC-II facility. SPICE features a permanent rare-earth magnetic lens to collect and direct internal conversion electrons emitted from nuclear reactions to a thick, highly segmented, lithium-drifted silicon detector. This arrangement, combined with TIGRESS, enables in-beam $\gamma$-ray and internal conversion electron spectroscopy to be performed with stable and radioactive ion beams. Technical aspects of the device, capabilities, and initial performance are presented.

Internal conversion coefficients have been measured for transitions in 110Pd to allow the determination of electric monopole (E0) transition strengths. Excited states were populated through inelastic alpha scattering and the SPICE+TIGRESS detectors at TRIUMF-ISAC-II were used to detect the emitted gamma rays and internal conversion electrons. The E0 transition strengths are found to be small and are consistent with the expectation for transitions from a K = 2 band to the K = 0 ground-state band in the axial rotor model.

Background: $\beta$-delayed multiple neutron emission has been observed for some nuclei with A$\leq$100, with $^{100}$Rb being the heaviest $\beta$2n emitter measured to date. So far, only 25 P$_{2n}$ values have been determined for the $\sim$300 nuclei that may decay in this way. Accordingly, it is of interest to measure P$_{2n}$ values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such measurement for nuclei with A$>$100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the $r$-process, and safety inputs for nuclear reactors. Purpose: To determine for the first time the two neutron branching ratio, P$_{2n}$ value, for $^{136}$Sb through a direct neutron measurement, and to provide precise P$_{1n}$ values for $^{136}$Sb and $^{136}$Te. Method: Pure beams were provided by the JYFLTRAP at the IGISOL facility of the University of Jyv\"askyl\"a, Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point, and the BELEN detector, based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the $\beta$- and neutron- growth-and-decay curves and the $\beta$-one-neutron and $\beta$-two-neutron time correlations. Results: The P$_{2n}$ value of $^{136}$Sb was found to be 0.31(5)\% and the measured P$_{1n}$ values for $^{136}$Sb and $^{136}$Te were found to be 31.9(15)\% and 1.47(6)\%, respectively. The measured P$_{2n}$ value is a factor 20 smaller than predicted by the FRDM+QRPA model used for $r$-process calculations.

Many-body nuclear theory utilizing microscopic or chiral potentials has developed to the point that collectivity might be dealt with in an {\it ab initio} framework without the use of effective charges; for example with the proper evolution of operators, or alternatively, through the use of an appropriate and manageable subset of particle-hole excitations. We present a precise determination of $E2$ strength in $^{22}$Mg and its mirror $^{22}$Ne by Coulomb excitation, allowing for rigorous comparisons with theory. No-core symplectic shell-model calculations were performed and agree with the new $B(E2)$ values while in-medium similarity-renormalization-group calculations consistently underpredict the absolute strength, with the missing strength found to have both isoscalar and isovector components., 7 pages, 5 figures. To be submitted to Physics Letters B

Background: The evolution of nuclear magic numbers at extremes of isospin is a topic at the forefront of contemporary nuclear physics. $N=50$ is a prime example, with increasing experimental data coming to light on potentially doubly magic $^{100}\mathrm{Sn}$ and $^{78}\mathrm{Ni}$ at the proton-rich and proton-deficient extremes, respectively; however, experimental discrepancies exist in the data for less exotic systems.Purpose: In $^{86}\mathrm{Kr}$ the $B(E2;{2}_{1}^{+}\ensuremath{\rightarrow}{0}_{1}^{+})$ value---a key indicator of shell evolution---has been experimentally determined by two different methodologies, with the results deviating by $3\ensuremath{\sigma}$. Here, we report on a new high-precision measurement of this value, as well as the first measured lifetimes and hence transition strengths for the ${2}_{2}^{+}$ and ${3}_{(2)}^{\ensuremath{-}}$ states in the nucleus.Methods: The Doppler-shift attenuation method was implemented using the TRIUMF-ISAC $\ensuremath{\gamma}$-ray escape-suppressed spectrometer (TIGRESS) $\ensuremath{\gamma}$-ray spectrometer and the TIGRESS integrated plunger device. High-statistics Monte Carlo simulations were utilized to extract lifetimes in accordance with state-of-the-art methodologies.Results: Lifetimes of $\ensuremath{\tau}({2}_{1}^{+})=336\ifmmode\pm\else\textpm\fi{}4\text{(stat.)}\ifmmode\pm\else\textpm\fi{}20\text{(sys.)}$ fs, $\ensuremath{\tau}({2}_{2}^{+})=263\ifmmode\pm\else\textpm\fi{}9\text{(stat.)}\ifmmode\pm\else\textpm\fi{}19\text{(sys.)}$ fs, and $\ensuremath{\tau}({3}_{(2)}^{\ensuremath{-}})=73\ifmmode\pm\else\textpm\fi{}6\text{(stat.)}\ifmmode\pm\else\textpm\fi{}32\text{(sys.)}$ fs were extracted. This yields a transition strength for the first-excited state of $B(E2;{2}_{1}^{+}\ensuremath{\rightarrow}{0}_{1}^{+})=259\ifmmode\pm\else\textpm\fi{}3\text{(stat.)}\ifmmode\pm\else\textpm\fi{}16\text{(sys.)}$ ${e}^{2}$ ${\mathrm{fm}}^{4}$.Conclusions: The measured lifetime disagrees with the previous Doppler-shift attenuation method measurement by more than $3\ensuremath{\sigma}$, while agreeing well with a previous value extracted from Coulomb excitation. The newly extracted $B(E2;{2}_{1}^{+}\ensuremath{\rightarrow}{0}_{1}^{+})$ value indicates a more significant reduction in the $N=50$ isotones approaching $Z=40$.

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter , a detection system sensitive to the implantation and decay of radioactive ions, and γ -ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and β -delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

A high-precision half-life measurement for the superallowed Fermi ${\ensuremath{\beta}}^{+}$ emitter $^{22}\mathrm{Mg}$ was performed at the TRIUMF-ISAC facility using a $4\ensuremath{\pi}$ proportional gas counter. The result of ${T}_{1/2}=3.87400\ifmmode\pm\else\textpm\fi{}0.00079$ s is a factor of 3 more precise than the previously adopted world average and resolves a discrepancy between the two previously published $^{22}\mathrm{Mg}$ half-life measurements.

The beta decays of 86Br and 91Rb have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the IGISOL facility in Jyvaskyla and further purified using the JYFLTRAP. 86Br and 91Rb are considered high priority contributors to the decay heat in reactors. In addition 91Rb was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam et al. assuming that this decay was well known from high-resolution measurements. Our results shows that both decays were suffering from the Pandemonium effect and that the results of Rudstam et al. should be renormalized.

Background: Previous measurements of Beta-delayed neutron emitters comprise around 230 nuclei, spanning from the 8He up to 150La. Apart from 210Tl, with a minuscule branching ratio of 0.07%, no other neutron emitter is measured yet beyond A = 150. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at A 195. Purpose: To measure both, Beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond N = 126. Method: Ions of interest are produced by fragmentation of a 238U beam, selected and identifed via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) is used to measure ion-implants and -decays. An array of 30 3He tubes embedded in a polyethylene matrix (BELEN) is used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time-correlations. The latter are analyzed with an analytical model and results for the half-lives and neutron-branching ratios are derived using the binned Maximum-Likelihood method. Results: Twenty new Beta-decay half-lives are reported for 204

The conceptual design of the BRIKEN neutron detector at the radioactive ion beam factory (RIBF) of the RIKEN Nishina Center is reported. The BRIKEN setup is a complex system aimed at detecting heavy-ion implants, ß particles, ¿ rays and ß-delayed neutrons. The whole setup includes the Advanced Implantation Detection Array (AIDA), two HPGe Clover detectors and up to 166 3He-filled counters embedded in a high-density polyethylene moderator. The design is quite complex due to the large number and different types of 3He-tubes involved and the additional constraints introduced by the ancillary detectors for charged particles and ¿ rays. This article reports on a novel methodology developed for the conceptual design and optimisation of the 3He-counter array, aiming for the best possible performance in terms of neutron detection. The algorithm is based on a geometric representation of two selected detector parameters of merit, namely, the average neutron detection efficiency and the efficiency flatness as a function of a reduced number of geometric variables. The response of the neutron detector is obtained from a systematic Monte Carlo simulation implemented in GEANT4. The robustness of the algorithm allowed us to design a versatile detection system, which operated in hybrid mode includes the full neutron counter and two clover detectors for high-precision gamma spectroscopy. In addition, the system can be reconfigured into a compact mode by removing the clover detectors and re-arranging the 3He tubes in order to maximize the neutron detection performance. Both operation modes shows a rather flat and high average efficiency. In summary, we have designed a system which shows an average efficiency for hybrid mode (3He tubes + clovers) of 68.6% and 64% for neutron energies up to 1 and 5 MeV, respectively. For compact mode (only 3He tubes), the average efficiency is 75.7% and 71% for neutron energies up to 1 and 5 MeV, respectively. The performance of the BRIKEN detection system has been also quantified by means of Monte Carlo simulations with different neutron energy distributions.

International audience; Total absorption gamma-ray spectroscopy is used to measure accurately the intensity of γ emission from neutron-unbound states populated in the β-decay of delayed-neutron emitters. From the comparison of this intensity with the intensity of neutron emission a constraint on the (n, γ) cross section for highly unstable neutron-rich nuclei can be deduced. A surprisingly large γ branching was observed for a number of isotopes which might indicate the need to increase by a large factor the Hauser-Feshbach (n, γ) cross-section estimates that impact on r process abundance calculations.

We investigate the decay of 87,88Br and 94Rb using total absorption γ -ray spectroscopy. These important fission products are β-delayed neutron emitters. Our data show considerable βγ intensity, so far unobserved in high-resolution γ -ray spectroscopy, from states at high excitation energy. We also find significant differences with the β intensity that can be deduced from existing measurements of the β spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235U fission at cooling times in the range 1–100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for γ emission from neutron unbound states populated in the daughter nucleus. The γ branching is compared to Hauser-Feshbach calculations, which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for 94Rb, although much smaller, hints of the need to increase the radiative width γ by one order of magnitude. This increase in γ would lead to a similar increase in the calculated (n,γ ) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations.

J. L. Taín et al. -- 6 pags., 7 figs., 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0, Total absorption gamma-ray spectroscopy is used to measure accurately the intensity of ¿ emission from neutron-unbound states populated in the ß-decay of delayed-neutron emitters. From the comparison of this intensity with the intensity of neutron emission one can deduce information on the (n,¿) cross section for unstable neutron-rich nuclei of interest in r process abundance calculations. A surprisingly large ¿ branching was observed for a number of isotopes. The results are compared with Hauser-Feshbach calculations and discussed., This work was supported by Spanish Ministerio de Economía y Competitividad under grants FPA2008-06419, FPA2010- 17142, FPA2011-24553, FPA2014-52823-C2-1-P, CPAN CSD- 2007-00042 (Ingenio2010) and the program Severo Ochoa (SEV-2014-0398). WG would like to thank the University of Valencia for support. This work was supported by the Academy of Finland under the Finnish Centre of Excellence Programme 2012-2017 (Project No. 21350). Work supported by EPSRC(UK) and STFC(UK) and the UK National Measurement Office. Work supported by the European Commission under the FP7/EURATOM contract 605203. FGK acknowledges support from the U.S. Department of Energy, under contract number DEAC02- 06CH11357.

Preliminary results from beta decay studies of nuclei that are important for reactor applications are presented. The beta decays have been studied using the total absorption technique (TAS) and the pure beams provided by the JYFLTRAP system at the IGISOL facility of the University of Jyväskylä. peerReviewed

Beta-delayed neutron emission (Beta-n) is a form of radioactive decay in which an electron, an anti-neutrino and one or more neutrons are emitted. This process arises if the energy window of the decay Q_Beta is greater than the neutron separation energy S n of the daughter. The probability in each decay of emitting neutrons is called the Pn value. This form of decay plays a key role in the synthesis of chemical elements in the Universe via the rapid neutron capture process, or r-process. The r-process proceeds far from the valley of nuclear stability, and leads to very neutron-rich nuclei that then decay to the line of stability. Most of these nuclei are ßn emitters. The initial abundance distribution is shaped by the decay half-life T1/2, but the neutron emission affects the final abundances in two ways: on the one hand it shifts the decay path to lower masses and on the other hand it provides a source of neutrons for late captures that will shift it in the opposite way. Thus, a good knowledge of Pn and T1/2 values of the nuclei between the line of stability and the r-process path is needed for a correct understanding of the observed abundances. Besides the astrophysical interest, the measurement of new Pn values and half-lives is also useful for refining nuclear structure models, constraining parameters of the models and testing ß-strength functions [3]. Our current understanding of the process of ß-delayed multiple neutron emission, as well as the competition between different open channels (gamma, one-neutron, two-neutron, etc), is incomplete because of the scarcity of experimental data. With these ideas in mind, the BRIKEN (Beta-delayed-neutron-measurements at RIKEN) collaboration was established, with the aim of greatly improving the quantity and quality of data the decays of very neutron-rich nuclei close to the r-process path.

An overview is given of our activities related to the study of the beta decay of neutron rich nuclei relevant for nuclear applications. Recent results of the study of the beta decay of 87,88 Br using a new segmented total absorption spectrometer are presented. The measurements were performed at the IGISOL facility using trap-assisted total absorption spectroscopy.

A new accurate determination of beta-delayed neutron emission probabilities from nuclei in the low mass region of the light fission group has been performed. The measurements were carried out using the BELEN 4π neutron counter at the IGISOL-JYFL mass separator in combination with a Penning trap. The new results significantly improve the uncertainties of neutron emission probabilities for {sup 91}Br, {sup 86}As, {sup 85}As, and {sup 85}Ge nuclei.

The energy distribution of the neutron background was measured for the first time at Hall A of the Canfranc Underground Laboratory. For this purpose we used a novel approach based on the combination of the information obtained with six large high-pressure 3 He proportional counters embedded in individual polyethylene blocks of different size. In this way not only the integral value but also the flux distribution as a function of neutron energy was determined in the range from 1 eV to 10 MeV. This information is of importance because different underground experiments show different neutron background energy dependence. The high sensitivity of the setup allowed to measure a neutron flux level which is about four orders of magnitude smaller that the neutron background at sea level. The integral value obtained is Φ Hall A = ( 3.44 ± 0.35 ) × 10 - 6 cm −2 s −1 .

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei (GRIFFIN) is a new high-efficiency $\gamma$-ray spectrometer for decay spectroscopy research with low-energy (20-60 keV) stopped radioactive beams from the Isotope Separator and Accelerator (ISAC) facility at TRIUMF in Vancouver, Canada. GRIFFIN is comprised of 16 HPGe clover detectors and hosts a suite of auxiliary detection systems for tagging $\beta$ particles, neutrons, and internal conversion electrons in coincidence with $\gamma$ rays. GRIFFIN is a powerful new tool for studying the nuclear structure of exotic short-lived isotopes far from stability, and for measuring weak $\gamma$-ray branches that are important in tests of fundamental symmetries and nuclear astrophysics. In this work, first results from the GRIFFIN physics program will be discussed, including a recent measurement of the half-lives of the neutron-rich $^{128-130}$Cd and $^{131}$In isotopes.

International audience; The accurate determination of reactor antineutrino spectra remains a very active research topic for which new methods of study have emerged in recent years. Indeed, following the long-recognized reactor anomaly (measured antineutrino deficit in short baseline reactor experiments when compared with spectral predictions), the three international reactor neutrino experiments Double Chooz, Daya Bay and Reno have recently demonstrated the existence of spectral distortions in their measurements with respect to the same predictions. These spectral predictions were obtained through the conversion of integral beta-energy spectra obtained at the ILL research reactor. Several studies have shown that the underlying nuclear physics required for the conversion of these spectra into antineutrino spectra is not totally understood. An alternative to such converted spectra is a complementary approach that consists of determining the antineutrino spectrum by means of the measurement and processing of nuclear data. The beta properties of some key fission products suffer from the pandemonium effect which can be circumvented by the use of the Total Absorption Gamma-ray Spectroscopy technique (TAGS). The two main contributors to the Pressurized Water Reactor antineutrino spectrum in the region where the spectral distortion has been observed are 92Rb and 142Cs, which have been measured at the radioactive beam facility of the University of Jyväskylä in two TAGS experiments. We present the results of the analysis of the TAGS measurements of the β-decay properties of 92Rb along with preliminary results on 142Cs and report on the measurements already performed.

The β-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with β-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N≳126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the β-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis.

The $\ensuremath{\beta}$-decay half-lives of $^{128--130}\mathrm{Cd}$ have been measured with the newly commissioned GRIFFIN $\ensuremath{\gamma}$-ray spectrometer at the TRIUMF-ISAC facility. The time structures of the most intense $\ensuremath{\gamma}$ rays emitted following the $\ensuremath{\beta}$ decay were used to determine the half-lives of $^{128}\mathrm{Cd}$ and $^{130}\mathrm{Cd}$ to be ${T}_{1/2}=246.2\phantom{\rule{0.16em}{0ex}}(21)$ ms and ${T}_{1/2}=126\phantom{\rule{0.16em}{0ex}}(4)$ ms, respectively. The half-lives of the $3/{2}^{+}$ and $11/{2}^{\ensuremath{-}}$ states of $^{129}\mathrm{Cd}$ were measured to be ${T}_{1/2}(3/{2}^{+})=157\phantom{\rule{0.16em}{0ex}}(8)$ ms and ${T}_{1/2}(11/{2}^{\ensuremath{-}})=147\phantom{\rule{0.16em}{0ex}}(3)$ ms. The half-lives of the Cd isotopes around the $N=82$ shell closure are an important ingredient in astrophysical simulations to derive the magnitude of the second $r$-process abundance peak in the $A\ensuremath{\sim}130$ region. Our new results are compared with recent literature values and theoretical calculations.

A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known β-delayed neutron emission properties. The setup consists of BELEN-20, a 4π neutron counter with twenty 3He proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for β counting and a self-triggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, β and β–neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on the accuracy of neutron emission probabilities is discussed. A new accurate value of the neutron emission probability for the important delayed-neutron precursor 137I was obtained, P n = 7.76 ( 14 ) %.