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Noise spectroscopy elucidates the fundamental noise sources in spin systems, which is essential for developing spin qubits with long coherence times for quantum information processing, communication, and sensing. But noise spectroscopy typically relies on microwave coherent spin control to extract the noise spectrum, which becomes infeasible when there are high-frequency noise components stronger than the available microwave power. Here, we demonstrate an alternative all-optical approach to performing noise spectroscopy. Our approach utilises coherent Raman rotations of the spin state with controlled timing and phase to implement Carr-Purcell-Meiboom-Gill (CPMG) pulse sequences. Analysing the spin dynamics under these sequences enables us to extract the noise spectrum of a dense ensemble of nuclear spins interacting with a single spin in a quantum dot, which has thus far only been modelled theoretically. By providing large spectral bandwidths of over 100 MHz, our Raman-based approach could serve as an important tool to study spin dynamics and decoherence mechanisms for a broad range of solid-state spin qubits.

Trapped ions are promising candidates for nodes of a scalable quantum network due to their long-lived qubit coherence times and high-fidelity single and two-qubit gates. Future quantum networks based on trapped ions will require a scalable way to route photons between different nodes. Photonic integrated circuits from fabrication foundries provide a compact solution to this problem. However, these circuits typically operate at telecommunication wavelengths which are incompatible with the strong dipole emissions of trapped ions. In this work, we demonstrate the routing of single photons from a trapped ion using a photonic integrated circuit. We employ quantum frequency conversion to match the emission of the ion to the operating wavelength of a foundry-fabricated silicon nitride photonic integrated circuit, achieving a total transmission of 31$\pm$0.9% through the device. Using programmable phase shifters, we switch the single photons between the output channels of the circuit and also demonstrate a 50/50 beam splitting condition. These results constitute an important step towards programmable routing and entanglement distribution in large-scale quantum networks and distributed quantum computers.

Atomic frequency combs memories that coherently store optical signals are a key building block for optical quantum computers1 and quantum networks2. Current atomic frequency combs typically use bulk materials or waveguides with large cross-sections3–5, or rely on fabrication techniques not easily adaptable to wafer scale processing6. Integrating such memories into compact and chip-scale devices is essential for scalable quantum technology. We demonstrate a compact chip-integrated atomic frequency comb in rare earth doped thin-film lithium niobate. Our optical memory exhibits a broad storage bandwidth exceeding 100 MHz, and optical storage time of over 250 ns. The enhanced optical confinement in this device leads to three orders of magnitude reduction in optical power required for coherent control as compared to ion-diffused waveguides 7. These compact atomic frequency comb memories pave the way towards scalable, highly efficient, electro-optically tunable quantum photonic systems that can store and manipulate light on a compact chip3.

Noise spectroscopy elucidates the fundamental noise sources in spin systems, which is essential for developing spin qubits with long coherence times for quantum information processing, communication, and sensing. But noise spectroscopy typically relies on microwave coherent spin control to extract the noise spectrum, which becomes infeasible when there are high-frequency noise components stronger than the available microwave power. Here, we demonstrate an alternative all-optical approach to performing noise spectroscopy. Our approach utilises coherent Raman rotations of the spin state with controlled timing and phase to implement Carr-Purcell-Meiboom-Gill (CPMG) pulse sequences. Analysing the spin dynamics under these sequences enables us to extract the noise spectrum of a dense ensemble of nuclear spins interacting with a single spin in a quantum dot, which has thus far only been modelled theoretically. By providing large spectral bandwidths of over 100 MHz, our Raman-based approach could serve as an important tool to study spin dynamics and decoherence mechanisms for a broad range of solid-state spin qubits.

Trapped ions form an advanced technology platform for quantum information processing with long qubit coherence times, high-fidelity quantum logic gates, optically active qubits, and a potential to scale up in size while preserving a high level of connectivity between qubits. These traits make them attractive not only for quantum computing but also for quantum networking. Dedicated, special-purpose trapped-ion processors in conjunction with suitable interconnecting hardware can be used to form quantum repeaters that enable high-rate quantum communications between distant trapped-ion quantum computers in a network. In this regard, hybrid traps with two distinct species of ions, where one ion species can generate ion-photon entanglement that is useful for optically interfacing with the network and the other has long memory lifetimes, useful for qubit storage, have been proposed for entanglement distribution. We consider an architecture for a repeater based on such dual-species trapped-ion systems. We propose and analyze a protocol based on spatial and temporal mode multiplexing for entanglement distribution across a line network of such repeaters. Our protocol offers enhanced rates compared to rates previously reported for such repeaters. We determine the ion resources required at the repeaters to attain the enhanced rates, and the best rates attainable when constraints are placed on the number of repeaters and the number of ions per repeater. Our results bolster the case for near-term trapped-ion systems as quantum repeaters for long-distance quantum communications., Comment: Published in Physical Review A

Radiative cascades emit correlated photon pairs, providing a pathway for the generation of entangled photons. The realization of a radiative cascade with impurity atoms in semiconductors, a leading platform for the generation of quantum light, would therefore provide a new avenue for the development of entangled photon pair sources. Here we demonstrate a radiative cascade from the decay of a biexciton at an impurity-atom complex in a ZnSe quantum well. The emitted photons show clear temporal correlations revealing the time--ordering of the cascade. Our result establishes impurity atoms in ZnSe as a potential platform for photonic quantum technologies using radiative cascades., Comment: 5 pages, 4 figures

Trapped ions excel as quantum networking nodes. Here, we use integrated photonic circuits to route and directionally switch single photons emitted by an ion. This is a key step towards scalable trapped ion quantum networks.

We demonstrate efficient fiber-interfacing photonic devices based on hole gratings producing a narrow directional beam that directly launch single photons from quantum dots into a standard single-mode fiber by matching the numerical aperture.

We experimentally demonstrate room temperature all-optical bistability at telecom wavelengths using a nanobeam photonic crystal cavity embedded with an ensemble of quantum dots. Reflectivity measurements are performed to confirm the thermo-optic nature of the bistability.

Defects in wide-bandgap semiconductors are promising qubit candidates for quantum communication and computation. Epitaxially grown II-VI semiconductors are particularly promising host materials due to their direct bandgap and potential for isotopic purification to a spin-zero nuclear background. Here, we show a new type of single photon emitter with potential electron spin qubit based on Cl impurities in ZnSe. We utilize a quantum well to increase the binding energies of donor emission and confirm single photon emission with short radiative lifetimes of 192 ps. Furthermore, we verify that the ground state of the Cl donor complex contains a single electron by observing two-electron satellite emission, leaving the electron in higher orbital states. We also characterize the Zeeman splitting of the exciton transition by performing polarization-resolved magnetic spectroscopy on single emitters. Our results suggest single Cl impurities are suitable as single photon source with potential photonic interface., Comment: 7 pages, 6 figures

Through multi-exciton cascade recombination in a quantum dot and engineered Purcell effect in a photonic crystal cavity, we demonstrate the single-photon emission with Gaussian-like spatial and temporal modes and temporally purify single photons from background emission.

We propose a quantum Fourier transform on photons in which a single atom-coupled cavity system mediates the photon-photon interactions. Our protocol utilizes time-delay feedback of photons and requires no active feedforward control. The time-delay feedback enables a single atom-cavity system to implement a quantum Fourier transform on an arbitrary number of photonic qubits on-the-fly, while rapid tuning of the atomic transition implements arbitrary controlled-phase gates. We analyze the performance of the protocol numerically and show that it can implement quantum Fourier transforms with tens of photons using state-of-the-art cavity quantum electrodynamics., 8 pages, 5 figures

Ultrathin optical limiters are needed to protect light sensitive components in miniaturized optical systems. However, it has proven challenging to achieve a sufficiently low optical limiting threshold. In this work, we theoretically show that an ultrathin optical limiter with low threshold intensity can be realized using a nonlinear zone plate. The zone plate is embedded with nonlinear saturable absorbing materials that allow the device to focus low intensity light, while high intensity light is transmitted as a plane wave without a focal spot. Based on this proposed mechanism, we use the finite-difference time-domain method to computationally design a zone plate embedded with InAs quantum dots as the saturable absorbing material. The device has a thickness of just 0.5 μm and exhibits good optical limiting behavior with a threshold intensity as low as 0.45 kW/cm2, which is several orders of magnitude lower than bulk limiter counterparts based on a similar mechanism, and also performs favorably compared to current ultrathin flat-optics-based optical limiters. This design can be optimized for different operating wavelengths and threshold intensities by using different saturable absorbing materials. Additionally, the diameter and focal length of the nonlinear zone plate can be easily adjusted to fit different systems and applications. Due to its flexible design, low power threshold, and ultrathin thickness, this optical limiting concept may be promising for application in miniaturized optical systems.

Integrated photonics is a powerful platform for future quantum technology that encodes and processes information using single photons. In this talk I will describe an experimental realization of a quantum transistor, which mediates strong interactions between single photons using a single semiconductor spin qubits. These interactions are a key requirement for active quantum photonic devices. I will also present our recent work on hybrid integration of these devices with photonics, as well as applications in photonic quantum computing and topological photonics.

Frequency conversion forms an integral block of the electronic circuits used in various applications including energy harvesting, communications and signal processing. These frequency conversion units however require external power sources and occupy a large device footprint making it difficult to be integrated in micro-circuits. Here we demonstrate that nanoscale magnetic tunnel junctions can act as frequency converters without an external power supply or DC bias source. The device directly mixes an external microwave signal with the internal spin precession oscillations to create new frequencies tunable by an external magnetic field in a single device with a small device footprint. We observe up-conversion and down-conversion of the input signal for excitation frequencies between 2 GHz and 6 GHz. We also show that the device acts as a zero-bias rectifier that can generate voltages exceeding 12 mV when the excitation frequency matches the natural oscillations mode of the device.

Action potentials are the basic unit of information in the nervous system, and their reliable detection and decoding holds the key to understanding how the brain generates complex thought and behavior. Transduction of these signals into microwave signal oscillations can enable wireless sensors that report on brain activity through magnetic induction. In this letter, we demonstrate that action potentials from the lateral giant neurons of crayfish can induce microwave oscillations in nanoscale magnetic tunnel junctions (NMTJs). We show that action potentials activate microwave oscillations in NMTJs with an amplitude that follows the action potential signal, demonstrating that the device has both the sensitivity and temporal resolution to respond to action potentials from a single neuron. The activation of magnetic oscillations by action potentials, together with the small surface area and the high-frequency tunability, makes these devices potential candidates for high-resolution sensing of bioelectric signals from neural tissues. These device attributes may be useful for the design of high-throughput bidirectional brain–machine interfaces.

We demonstrate a low power thermally induced optical bistability at telecom wavelengths and room temperature using a nanobeam photonic crystal cavity embedded with an ensemble of quantum dots. The nanobeam photonic crystal cavity is transfer-printed onto the edge of a carrier chip for thermal isolation of the cavity with an efficient optical coupling between the nanobeam waveguide and optical setup. Reflectivity measurements performed with a tunable laser reveal the thermo-optic nature of the nonlinearity. A bistability power threshold as low as 23 μW and an on/off response contrast of 6.02 dB are achieved from a cavity with a moderately low quality factor of 2830. Our device provides optical bistability at power levels an order of magnitude lower than previous quantum-dot-based devices.

We introduce an all-optical approach for noise spectroscopy of solid-state spin qubits, based on Raman control and the Carr-Purcell-Meiboom-Gill pulse sequences, and use it to extract the noise spectra of self-assembled quantum dots.

Topological photonic structures exhibit chiral edge states that are robust to disorder and sharp bends. When coupled to quantum emitters, these edge states generate directional light emission that enables unprecedented control of interactions between light and matter in a nanophotonic device. While directional light emission in one-dimensional topological, as well as conventional, waveguides has been previously demonstrated, the extension of these concepts to resonator structures that enhance light-matter coupling remains challenging. Here we demonstrate chiral lightmatter interactions in a topological resonator. We employ valley-Hall topological edge states to realize a helical resonator at the interface of two topologically distinct regions. Such a helical resonator has two counter-propagating modes with opposite polarizations. We show chiral coupling of the resonator to a quantum emitter resulting in a Purcell enhancement of 3.4 due to resonant coupling. Such chiral resonators could enable designing complex nanophotonic circuits for quantum information processing, and studying novel quantum many-body dynamics.

Bright fiber-coupled single photon sources are essential components for practical quantum network. In this work, we present a bright single photon source based on an InAs/InP quantum dot emitting at telecom wavelengths. We designed a nanobeam with a photonic crystal mirror at the other end and a tapered coupler at the other end enabling both directional emission and gaussian-like far-field profile. We detected fiber-coupled single photon count rate of 1.1 MHz with 40 MHz pumping rate. Considering losses from optics and spectral filters, we achieved collection efficiency into first lens of 68% and a total fiber collection efficiency of 8.2%.

Here we demonstrate chiral light-matter interactions in a topological photonic crystal resonator. We achieve this by employing valley-Hall topological edge states to create a helical resonator at the interface of two topologically distinct regions.

The efficient single photon emission capabilities of quantum dot molecules position them as promising platforms for quantum information processing. Furthermore, quantum dot molecules feature a "decoherence-free" subspace that enables spin qubits with long coherence time. To efficiently read out the spin state within this subspace requires optically cycling isolated transitions that originate from a triplet manifold within the quantum dot molecule. We propose and theoretically study a two-stage spin readout protocol within this decoherence-free subspace that allows single-shot readout performance. The process incorporates a microwave $\pi$-pulse and optically cycling the isolated transitions, which induces fluorescence that allows us to identify the initial spin state. This protocol offers enhanced readout fidelity compared to previous schemes that rely on the excitation of transitions that strongly decay to multiple ground states or require long initialization via slow, optically forbidden transitions. By simulating the performance of the protocol, we show that an optimal spin readout fidelity of over 97% and single-shot readout performance are achievable for a photon collection efficiency of just 0.12%. This high readout performance for such realistic photon collection conditions within the decoherence-free subspace expands the potential of quantum dot molecules as building blocks for quantum networks.

We demonstrate single photon emission from donor bound excitons in Cl doped ZnSe quantum wells. The emitters are investigated in cryogenic temperatures, and they showed high binding energies and short lifetimes.

Future scalable photonic quantum information processing relies on the ability of integrating multiple interacting quantum emitters into a single chip. Quantum dots provide ideal on-chip quantum light sources. However, achieving quantum interaction between multiple quantum dots on-a-chip is a challenging task due to the randomness in their frequency and position, requiring local tuning technique and long-range quantum interaction. Here, we demonstrate quantum interactions between distant two quantum dots on a nanophotonic waveguide. We achieve a photon-mediated long-range interaction by integrating the quantum dots to the same optical mode of a nanophotonic waveguide and overcome spectral mismatch by incorporating on-chip thermal tuners. We observe their quantum interactions of the form of super-radiant emission, where the two dots collectively emit faster than each dot individually. Creating super-radiant emission from integrated quantum emitters could enable compact chip-integrated photonic structures that exhibit long-range quantum interactions. Therefore, these results represent a major step towards establishing photonic quantum information processors composed of multiple interacting quantum emitters on a semiconductor chip., Comment: 23 pages, 7 figures

Hybrid organic–inorganic perovskites containing Cs are a promising new material for light-absorbing and light-emitting optoelectronics. However, the impact of environmental conditions on their optical properties is not fully understood. Here, we elucidate and quantify the influence of distinct humidity levels on the charge carrier recombination in CsxFA1–xPb(IyBr1–y)3 perovskites. Using in situ environmental photoluminescence (PL), we temporally and spectrally resolve light emission within a loop of critical relative humidity (rH) levels. Our measurements show that exposure up to 35% rH increases the PL emission for all Cs (10–17%) and Br (17–38%) concentrations investigated here. Spectrally, samples with larger Br concentrations exhibit PL redshift at higher humidity levels, revealing water-driven halide segregation. The compositions considered present hysteresis in their PL intensity upon returning to a low-moisture environment due to partially reversible hydration of the perovskites. Our findings demon...

Fiber-based quantum networks require photons at telecommunications wavelengths to interconnect qubits separated by long distances. Trapped ions are leading candidates for quantum networking with high-fidelity two-qubit gates, long coherence times, and the ability to readily emit photons entangled with the ion's internal qubit states. However, trapped ions typically emit photons at wavelengths incompatible with telecommunications fiber. Here, we demonstrate frequency conversion of visible photons, emitted from the S-P dipole transition of a trapped Ba+ ion, into the telecommunications C-band. These results are an important step towards enabling a long-distance trapped ion quantum internet.

The majority of photonic quantum information technologies rely on single photons that have high purity and indistinguishability. Although solid-state quantum emitters can serve such single photons on demand, their asymmetric temporal and spatial mode profiles limit the optimal efficiency and fidelity of quantum interaction. Here, we demonstrate single-photon pulses at a telecom wavelength with a Gaussian-like temporal mode profile from a cavity-coupled single quantum dot. Engineering the exciton dynamics via multi-exciton cascade recombination and cavity detuning enables us to modify the rise and decay dynamics of single excitons. Furthermore, the cascade recombination process temporally retards the single-exciton emission from the background emission, leading to possible purification of single photons at high excitation power. In addition, coupling quantum dots into a low Q cavity mode leads to a Gaussian-like spatial mode profile, which brings a high collection efficiency. This approach paves the way for producing single photons with an optimized temporal and spatial waveform.

In this work, we demonstrate a transferrable single crystalline 4H-SiC nanomembrane (SiC NM) released from a SiC-on-insulator (SiCOI) wafer. High resolution X-ray diffraction (XRD) and atomic force microscopy (AFM) were performed on the SiC NM and confirmed similarly good crystallinity and surface morphology. In addition, the refractive index and extinction coefficient of the SiC NM were investigated using ellipsometry analyses. Despite its thinness (i.e., 200 nm), the SiC NM achieved an absorption greater than 40% in the wavelength range of 200–260 nm with a maximum absorption of 73.8% at 256 nm. Our transferrable SiC NM provides not only good mechanical flexibility, but also exhibits excellent ultraviolet (UV) light absorption which could be readily utilized for high sensitivity flexible UV detectors.

Devices known as quantum cascade lasers produce useful terahertz radiation, but are typically highly sensitive to fabrication defects. This limitation has now been overcome using a property called topological robustness. Terahertz radiation from a topological laser.

Charged quantum dots containing an electron or hole spin are bright solid-state qubits suitable for quantum networks and distributed quantum computing. Incorporating such quantum dot spin into a photonic crystal cavity creates a strong spin-photon interface, in which the spin can control a photon by modulating the cavity reflection coefficient. However, previous demonstrations of such spin-photon interfaces have relied on quantum dots that are charged randomly by nearby impurities, leading to instability in the charge state, which causes poor contrast in the cavity reflectivity. Here we demonstrate a strong spin-photon interface using a quantum dot that is charged deterministically with a diode structure. By incorporating this actively charged quantum dot in a photonic crystal cavity, we achieve strong coupling between the cavity mode and the negatively charged state of the dot. Furthermore, by initializing the spin through optical pumping, we show strong spin-dependent modulation of the cavity reflectivity, corresponding to a cooperativity of 12. This spin-dependent reflectivity is important for mediating entanglement between spins using photons, as well as generating strong photon-photon interactions for applications in quantum networking and distributed quantum computing.

Integration of single-photon sources and detectors to silicon-based photonics opens the possibility of complex circuits for quantum information processing. In this work, we demonstrate integration of quantum dots with a silicon photonic add-drop filter for on-chip filtering and routing of telecom single photons. A silicon microdisk resonator acts as a narrow filter that transfers the quantum dot emission and filters the background over a wide wavelength range. Moreover, by tuning the quantum dot emission wavelength over the resonance of the microdisk we can control the transmission of the emitted single photons to the drop and through channels of the add-drop filter. This result is a step toward the on-chip control of single photons using silicon photonics for applications in quantum information processing, such as linear optical quantum computation and boson sampling.

Temporal multiplexing provides an efficient and scalable approach to realize a quantum random walk with photons that can exhibit topological properties. But two-dimensional time-multiplexed topological quantum walks studied so far have relied on generalizations of the Su-Shreiffer-Heeger model with no synthetic gauge field. In this work, we demonstrate a two-dimensional topological quantum random walk where the nontrivial topology is due to the presence of a synthetic gauge field. We show that the synthetic gauge field leads to the appearance of multiple band gaps and, consequently, a spatial confinement of the quantum walk distribution. Moreover, we demonstrate topological edge states at an interface between domains with opposite synthetic fields. Our results expand the range of Hamiltonians that can be simulated using photonic quantum walks.

Rare-earth ion ensembles doped in single crystals are a promising materials system with widespread applications in optical signal processing, lasing, and quantum information processing. Incorporating rare-earth ions into integrated photonic devices could enable compact lasers and modulators, as well as on-chip optical quantum memories for classical and quantum optical applications. To this end, a thin film single crystalline wafer structure that is compatible with planar fabrication of integrated photonic devices would be highly desirable. However, incorporating rare-earth ions into a thin film form-factor while preserving their optical properties has proven challenging. We demonstrate an integrated photonic platform for rare-earth ions doped in a single crystalline thin film on insulator. The thin film is composed of lithium niobate doped with Tm3+. The ions in the thin film exhibit optical lifetimes identical to those measured in bulk crystals. We show narrow spectral holes in a thin film waveguide that require up to 2 orders of magnitude lower power to generate than previously reported bulk waveguides. Our results pave way for scalable on-chip lasers, optical signal processing devices, and integrated optical quantum memories.

The goal of integrated quantum photonics is to combine components for the generation, manipulation, and detection of non-classical light in a phase stable and efficient platform. Solid-state quantum emitters have recently reached outstanding performance as single photon sources. In parallel, photonic integrated circuits have been advanced to the point that thousands of components can be controlled on a chip with high efficiency and phase stability. Consequently, researchers are now beginning to combine these leading quantum emitters and photonic integrated circuit platforms to realize the best properties of each technology. In this article, we review recent advances in integrated quantum photonics based on such hybrid systems. Although hybrid integration solves many limitations of individual platforms, it also introduces new challenges that arise from interfacing different materials. We review various issues in solid-state quantum emitters and photonic integrated circuits, the hybrid integration techniques that bridge these two systems, and methods for chip-based manipulation of photons and emitters. Finally, we discuss the remaining challenges and future prospects of on-chip quantum photonics with integrated quantum emitters., Comment: 17 pages, 9 figures

In this paper, we have developed a method for describing the dynamics of an arbitrary quantum system under a bidirectional time-delayed feedback loop. For this purpose, we have described the evolution in terms of the time propagation of the quantum system of interest without feedback together with several identical systems, which represent the history of the quantum system under study. This technique provides a numerically efficient solution for describing a system's dynamics in the case of significant time delays in which direct investigation of the state of the reservoirs becomes numerically intractable. Using this method, we have studied two scenarios of multiple scatterings of photons incident on a cavity with a two-level atom positioned inside it, coupled to two waveguides that are connected at their ends. In the first scenario, two photons impinge on the cavity through separate waveguides with a delay between them. We have demonstrated that the maximum difference between the two output photon numbers occurs when the delay between the incident photons becomes close to the inverse of their linewidth. In the second scenario, multiple photons impinge on the cavity through the same waveguide and go through multiple interactions. We have shown that, for a fixed atom-cavity coupling rate, the transmission rate enhances as the number of photons increases and have quantified this enhancement. The developed method enables us to study a broad range of nonlinear dynamics in complex quantum networks.